Simulation of time- and frequency-resolved four-wave-mixing signals at finite temperatures: a thermo-field dynamics approach

• Main Authors: Chen, Lipeng, Borrelli, Raffaele, Shalashilin, Dmitrii V., Zhao, Yang, Gelin, Maxim F.
• 其他作者: School of Materials Science and Engineering
• 格式: Article
• 語言: English
• 出版: 2022
• 主題: Science::Chemistry; Fluorescence; Correlation Function
• 在線閱讀: https://hdl.handle.net/10356/157805

We propose a new approach to simulate four-wave-mixing signals of molecular systems at finite temperatures by combining the multiconfigurational Ehrenfest method with the thermo-field dynamics theory. In our approach, the four-time correlation functions at finite temperatures are mapped onto those a...