Time-dependent wave packet averaged vibrational frequencies from femtosecond stimulated Raman spectra
Femtosecond stimulated Raman spectroscopy (FSRS) on the Stokes side arises from a third order polarization, P(3)(t), which is given by an overlap of a first order wave packet, |||Ψ(1)2(pu,t)⟩Ψ2(1)(pu,t), prepared by a narrow band (ps) Raman pump pulse, Epu(t), on the upper electronic e2 potential en...
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語言: | English |
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2017
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在線閱讀: | https://hdl.handle.net/10356/86606 http://hdl.handle.net/10220/44129 |
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