Dynamics of the Davydov D-squared Ansatz with off-diagonal coupling
Following the Dirac-Frenkel time-dependent variational principle, dynamics of a one-dimensional Holstein polaron with off-diagonal exciton-phonon coupling is probed by employing the Davy dov D2 Ansatz with two sets of variational parameters,one for each constituting particle in the exciton-phonon sy...
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| Main Authors: | , , |
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| 格式: | Article |
| 語言: | English |
| 出版: |
2011
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| 在線閱讀: | https://hdl.handle.net/10356/93836 http://hdl.handle.net/10220/6784 |
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| 總結: | Following the Dirac-Frenkel time-dependent variational principle, dynamics of a one-dimensional Holstein polaron with off-diagonal exciton-phonon coupling is probed by employing the Davy dov D2 Ansatz with two sets of variational parameters,one for each constituting particle in the exciton-phonon system. A close examination of variational outputs from the two trial states reveals fine details of the polar on structure and intricacies of dynamic exciton-phonon interactions. Superradiance coherence sizes, speeds of exciton-induced phonon wave packets, linear optical absorption, and polaron energy compositions are also included in the study. |
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