Low threshold, amplified spontaneous emission from core-seeded semiconductor nanotetrapods incorporated into a sol-gel matrix

Wet-chemically synthesized CdSe seeded CdS nanotetrapods incorporated into silica matrices have been explored as high performance nanocrystal-based optical amplifiers. Varying the physical dimensions of the tetrapods allowed for room temperature biexcitonic amplified spontaneous emission (ASE) at wa...

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Main Authors: Liao, Yile, Xing, Guichuan, Mishra, Nimai, Sum, Tze Chien, Chan, Yinthai
其他作者: School of Physical and Mathematical Sciences
格式: Article
語言:English
出版: 2013
在線閱讀:https://hdl.handle.net/10356/97461
http://hdl.handle.net/10220/10665
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總結:Wet-chemically synthesized CdSe seeded CdS nanotetrapods incorporated into silica matrices have been explored as high performance nanocrystal-based optical amplifiers. Varying the physical dimensions of the tetrapods allowed for room temperature biexcitonic amplified spontaneous emission (ASE) at wavelengths corresponding to either the CdSe core or CdS arms, while higher pump intensities resulted in ASE from a higher CdSe excited state. These results collectively indicate that such heterostructured tetrapods can facilitate tunable, multiple-wavelength lasing across a wide spectral range from a single nanostructure.