Selective excitation of atomic-scale dynamics by coherent exciton motion in the non-born–Oppenheimer regime

• Main Authors: Nie, Zhaogang., Long, Run., Li, Jialin., Zheng, Yi Ying., Prezhdo, Oleg V., Loh, Zhi-Heng.
• Other Authors: School of Physical and Mathematical Sciences
• Format: Article
• Language: English
• Published: 2014
• Subjects: DRNTU::Science::Chemistry::Physical chemistry
• Online Access: https://hdl.handle.net/10356/101655; http://hdl.handle.net/10220/18680
• Institution: Nanyang Technological University

Time-domain investigations of the nonadiabatic coupling between electronic and vibrational degrees of freedom have focused primarily on the formation of electronic superpositions induced by atomic motion. The effect of electronic nonstationary-state dynamics on atomic motion remains unexplored. H...