Temperature-dependent ultrafast carrier and phonon dynamics of topological insulator Bi1.5Sb0.5Te1.8Se1.2

Using ultrafast optical pump-probe technique, we studied the temperature-dependent carrier and phonon dynamics of the topological insulator Bi1.5Sb0.5Te1.8Se1.2 single-crystal from 10 K to 300 K. Two relaxation processes of carriers and coherent optical/acoustic phonons have been observed. By using...

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Bibliographic Details
Main Authors: Cheng, Liang, La-o-vorakiat, Chan, Tang, Chi Sin, Nair, Saritha K., Xia, Bin, Wang, Lan, Zhu, Jian-Xin, Chia, Elbert E. M.
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2014
Subjects:
Online Access:https://hdl.handle.net/10356/103713
http://hdl.handle.net/10220/20019
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Institution: Nanyang Technological University
Language: English
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Summary:Using ultrafast optical pump-probe technique, we studied the temperature-dependent carrier and phonon dynamics of the topological insulator Bi1.5Sb0.5Te1.8Se1.2 single-crystal from 10 K to 300 K. Two relaxation processes of carriers and coherent optical/acoustic phonons have been observed. By using the two-temperature model, we are able to attribute the fast (∼ps) relaxation component to carrier-phonon coupling involving carriers in the conduction band. We also studied the temperature dependence of the dephasing time and frequency of optical phonon, and the optical penetration depth of Bi1.5Sb0.5Te1.8Se1.2.