Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath

An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the c...

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Main Authors: Liu, Jing, Sun, Kewei, Wang, Xiaoguang, Zhao, Yang
Other Authors: School of Materials Science & Engineering
Format: Article
Language:English
Published: 2015
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Online Access:https://hdl.handle.net/10356/106709
http://hdl.handle.net/10220/25128
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1067092023-07-14T15:46:12Z Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath Liu, Jing Sun, Kewei Wang, Xiaoguang Zhao, Yang School of Materials Science & Engineering DRNTU::Science::Physics::Atomic physics::Quantum theory An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the coupling strength on the non-Markovian behavior of the chromophore in a super-Ohmic bath. It is found that an increase in the temperature results in a reduction in the backflow information from the environment to the chromophore, and therefore, a suppression of non-Markovianity. In the weak coupling regime, increasing coupling strength will enhance the non-Markovianity, while the effect is reversed in the strong coupling regime. Accepted version 2015-02-27T01:27:23Z 2019-12-06T22:16:36Z 2015-02-27T01:27:23Z 2019-12-06T22:16:36Z 2015 2015 Journal Article Liu, J., Sun, K., Wang, X., & Zhao, Y. (2015). Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath. Physical chemistry chemical physics, in press. https://hdl.handle.net/10356/106709 http://hdl.handle.net/10220/25128 10.1039/C4CP04922E en Physical chemistry chemical physics © 2015 The Authors. This is the author created version of a work that has been peer reviewed and accepted for publication in Physical Chemistry Chemical Physics, published by Royal Society of Chemistry on behalf of The Authors. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [Article URL/DOI: http://dx.doi.org/10.1039/C4CP04922E]. 11 p. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic DRNTU::Science::Physics::Atomic physics::Quantum theory
spellingShingle DRNTU::Science::Physics::Atomic physics::Quantum theory
Liu, Jing
Sun, Kewei
Wang, Xiaoguang
Zhao, Yang
Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
description An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the coupling strength on the non-Markovian behavior of the chromophore in a super-Ohmic bath. It is found that an increase in the temperature results in a reduction in the backflow information from the environment to the chromophore, and therefore, a suppression of non-Markovianity. In the weak coupling regime, increasing coupling strength will enhance the non-Markovianity, while the effect is reversed in the strong coupling regime.
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Liu, Jing
Sun, Kewei
Wang, Xiaoguang
Zhao, Yang
format Article
author Liu, Jing
Sun, Kewei
Wang, Xiaoguang
Zhao, Yang
author_sort Liu, Jing
title Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
title_short Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
title_full Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
title_fullStr Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
title_full_unstemmed Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath
title_sort quantifying non-markovianity for a chromophore-qubit pair in a super-ohmic bath
publishDate 2015
url https://hdl.handle.net/10356/106709
http://hdl.handle.net/10220/25128
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