A dopant‐free polymer as hole‐transporting material for highly efficient and stable perovskite solar cells

A series of thiazolothiazole‐thiophene‐based polymer hole‐transporting materials (HTMs) are synthesized and applied into perovskite solar cells (PSCs). These polymer HTMs have good performance and stability without any dopants. The improved performance and stability of PSCs is attributed to the poly...

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Bibliographic Details
Main Authors: Li, Xianqiang, Tang, Xiaohong, Yang, Yijie, Ye, Tao, Wu, Dan, Wang, Hong, Li, Jun, Wang, Xizu
Other Authors: School of Electrical and Electronic Engineering
Format: Article
Language:English
Published: 2020
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Online Access:https://hdl.handle.net/10356/136641
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Institution: Nanyang Technological University
Language: English
Description
Summary:A series of thiazolothiazole‐thiophene‐based polymer hole‐transporting materials (HTMs) are synthesized and applied into perovskite solar cells (PSCs). These polymer HTMs have good performance and stability without any dopants. The improved performance and stability of PSCs is attributed to the polymer HTMs' crystallinity which can be controlled by adjusting the thiophene units on the polymer backbone. The highest PCE of the polymer HTMs based PSCs reached 14.02%. The stability of the PSCs was shown by retaining 80% PCE of the original value after stored them in a N2‐filled glovebox for 113 days.