Dynamic response of magnetic skyrmions in multilayer heterostructures

Topological effects in condensed matter physics have been explored for fundamental and technological reasons in a wide variety of materials. Recently, magnetic skyrmions - circularly-shaped twisted spin textures - have aroused interest due to their enhanced stability and efficient coupling with elec...

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Main Author: Satywali, Bhartendu
Other Authors: Christos Panagopoulos
Format: Thesis-Doctor of Philosophy
Language:English
Published: Nanyang Technological University 2020
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Online Access:https://hdl.handle.net/10356/137378
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spelling sg-ntu-dr.10356-1373782023-02-28T23:58:07Z Dynamic response of magnetic skyrmions in multilayer heterostructures Satywali, Bhartendu Christos Panagopoulos School of Physical and Mathematical Sciences christos@ntu.edu.sg Science::Physics Topological effects in condensed matter physics have been explored for fundamental and technological reasons in a wide variety of materials. Recently, magnetic skyrmions - circularly-shaped twisted spin textures - have aroused interest due to their enhanced stability and efficient coupling with electric currents. Consequently, they can be harnessed for data storage and logic operations. Two key requirements for skyrmion formation are (a) an absence of spatial inversion symmetry and (b) a large spin-orbit coupling in the material. Metallic multilayers featuring ferromagnet-heavy metal (FM-HM) interfaces satisfy both conditions and can hence exhibit nano-skyrmions at room temperature (RT). In this thesis, we nucleate sub-50 nm skyrmions at RT in engineered Ir/Fe/Co/Pt multilayers, where the size and order (lattice or isolated) of the skyrmions can be tuned by the relative thickness of the Fe/Co layers. We employ magnetic force microscopy (MFM) to image skyrmions at RT. A significant variation is observed in the size and shape of skyrmions in different regions of the film, suggesting local inhomogeneities in the magnetic parameters for our films. A detailed analysis of the microwave excitation modes of skyrmions is of profound importance for understanding their current and field-induced dynamics. In this thesis, we report the first experimental detection of magnetic resonance from Neel skyrmions in multilayers from 300K-100K, measured with a home-built broadband ferromagnetic resonance (FMR) probe. The field and frequency-sweep FMR measurements reveal two distinct resonant modes originating from skyrmions: a low frequency (LF) resonance exhibiting a steep proportionality to the external out-of-plane magnetic field (H), and a high frequency (HF) resonance which is less sensitive to variations in H. Combining micromagnetic simulations and analytical calculations, we identify the counterclockwise (CCW) skyrmion gyrations to be responsible for the LF mode. The HF mode is caused by the scattering of magnons from the uniformly-precessing ferromagnetic background off skyrmions. Furthermore, we present a method of tuning the skyrmion excitation frequencies by varying the thickness of the non-magnetic Pt/Ir spacer layers in our heterostructures, which modulates the dipolar coupling between the FM layers. Doctor of Philosophy 2020-03-19T02:45:57Z 2020-03-19T02:45:57Z 2020 Thesis-Doctor of Philosophy Satywali, B. (2020). Dynamic response of magnetic skyrmions in multilayer heterostructures. Doctoral thesis, Nanyang Technological University, Singapore. https://hdl.handle.net/10356/137378 10.32657/10356/137378 en This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License (CC BY-NC 4.0). application/pdf Nanyang Technological University
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
spellingShingle Science::Physics
Satywali, Bhartendu
Dynamic response of magnetic skyrmions in multilayer heterostructures
description Topological effects in condensed matter physics have been explored for fundamental and technological reasons in a wide variety of materials. Recently, magnetic skyrmions - circularly-shaped twisted spin textures - have aroused interest due to their enhanced stability and efficient coupling with electric currents. Consequently, they can be harnessed for data storage and logic operations. Two key requirements for skyrmion formation are (a) an absence of spatial inversion symmetry and (b) a large spin-orbit coupling in the material. Metallic multilayers featuring ferromagnet-heavy metal (FM-HM) interfaces satisfy both conditions and can hence exhibit nano-skyrmions at room temperature (RT). In this thesis, we nucleate sub-50 nm skyrmions at RT in engineered Ir/Fe/Co/Pt multilayers, where the size and order (lattice or isolated) of the skyrmions can be tuned by the relative thickness of the Fe/Co layers. We employ magnetic force microscopy (MFM) to image skyrmions at RT. A significant variation is observed in the size and shape of skyrmions in different regions of the film, suggesting local inhomogeneities in the magnetic parameters for our films. A detailed analysis of the microwave excitation modes of skyrmions is of profound importance for understanding their current and field-induced dynamics. In this thesis, we report the first experimental detection of magnetic resonance from Neel skyrmions in multilayers from 300K-100K, measured with a home-built broadband ferromagnetic resonance (FMR) probe. The field and frequency-sweep FMR measurements reveal two distinct resonant modes originating from skyrmions: a low frequency (LF) resonance exhibiting a steep proportionality to the external out-of-plane magnetic field (H), and a high frequency (HF) resonance which is less sensitive to variations in H. Combining micromagnetic simulations and analytical calculations, we identify the counterclockwise (CCW) skyrmion gyrations to be responsible for the LF mode. The HF mode is caused by the scattering of magnons from the uniformly-precessing ferromagnetic background off skyrmions. Furthermore, we present a method of tuning the skyrmion excitation frequencies by varying the thickness of the non-magnetic Pt/Ir spacer layers in our heterostructures, which modulates the dipolar coupling between the FM layers.
author2 Christos Panagopoulos
author_facet Christos Panagopoulos
Satywali, Bhartendu
format Thesis-Doctor of Philosophy
author Satywali, Bhartendu
author_sort Satywali, Bhartendu
title Dynamic response of magnetic skyrmions in multilayer heterostructures
title_short Dynamic response of magnetic skyrmions in multilayer heterostructures
title_full Dynamic response of magnetic skyrmions in multilayer heterostructures
title_fullStr Dynamic response of magnetic skyrmions in multilayer heterostructures
title_full_unstemmed Dynamic response of magnetic skyrmions in multilayer heterostructures
title_sort dynamic response of magnetic skyrmions in multilayer heterostructures
publisher Nanyang Technological University
publishDate 2020
url https://hdl.handle.net/10356/137378
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