Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques
Renewable energy conversion and storage play an important role in our global efforts to limit the drastic effects of climate change. In particular, the electrocatalytic reduction of carbon dioxide to chemicals and fuels can bring us closer towards a closed-loop anthropogenic carbon cycle. Significan...
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sg-ntu-dr.10356-1388412020-06-01T10:26:46Z Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques Handoko, Albertus D. Wei, Fengxia Jenndy Yeo, Boon Siang Seh, Zhi Wei School of Materials Science & Engineering Engineering::Materials Characterization and Analytical Techniques Electrocatalysis Renewable energy conversion and storage play an important role in our global efforts to limit the drastic effects of climate change. In particular, the electrocatalytic reduction of carbon dioxide to chemicals and fuels can bring us closer towards a closed-loop anthropogenic carbon cycle. Significant breakthroughs are often the result of deeper understandings of reaction mechanisms, material structures and surface sites. To this end, operando techniques have been invaluable in combining advanced characterization of a catalyst with simultaneous measurements of its activity and selectivity under real working conditions. This Review aims to highlight significant progress in the use of operando characterization techniques that enhance our understanding of heterogeneous electrocatalytic CO 2 reduction. We provide a summary of the most recent mechanistic understanding using operando optical, X-ray and electron-based techniques, along with key questions that need to be addressed. We conclude by offering some insight on emerging directions and prospects in the field. ASTAR (Agency for Sci., Tech. and Research, S’pore) 2020-05-13T05:26:16Z 2020-05-13T05:26:16Z 2018 Journal Article Handoko, A. D., Wei, F., Jenndy, Yeo, B. S., & Seh, Z. W. (2018). Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques. Nature Catalysis, 1(12), 922-934. doi:10.1038/s41929-018-0182-6 2520-1158 https://hdl.handle.net/10356/138841 10.1038/s41929-018-0182-6 2-s2.0-85058512388 12 1 922 934 en Nature Catalysis © 2018 Springer Nature Limited. All rights reserved. |
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Engineering::Materials Characterization and Analytical Techniques Electrocatalysis Handoko, Albertus D. Wei, Fengxia Jenndy Yeo, Boon Siang Seh, Zhi Wei Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
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Renewable energy conversion and storage play an important role in our global efforts to limit the drastic effects of climate change. In particular, the electrocatalytic reduction of carbon dioxide to chemicals and fuels can bring us closer towards a closed-loop anthropogenic carbon cycle. Significant breakthroughs are often the result of deeper understandings of reaction mechanisms, material structures and surface sites. To this end, operando techniques have been invaluable in combining advanced characterization of a catalyst with simultaneous measurements of its activity and selectivity under real working conditions. This Review aims to highlight significant progress in the use of operando characterization techniques that enhance our understanding of heterogeneous electrocatalytic CO 2 reduction. We provide a summary of the most recent mechanistic understanding using operando optical, X-ray and electron-based techniques, along with key questions that need to be addressed. We conclude by offering some insight on emerging directions and prospects in the field. |
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School of Materials Science & Engineering |
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School of Materials Science & Engineering Handoko, Albertus D. Wei, Fengxia Jenndy Yeo, Boon Siang Seh, Zhi Wei |
format |
Article |
author |
Handoko, Albertus D. Wei, Fengxia Jenndy Yeo, Boon Siang Seh, Zhi Wei |
author_sort |
Handoko, Albertus D. |
title |
Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
title_short |
Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
title_full |
Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
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Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
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Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
title_sort |
understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques |
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2020 |
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https://hdl.handle.net/10356/138841 |
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1681057836327501824 |