Advances in small perovskite-based lasers

Lead halide perovskites have recently become a rapidly growing research field due to their great potential in next‐generation solar cells and photonic sources. As a direct bandgap semiconductor, perovskites are also promising candidates for low‐threshold and multicolor lasing devices due to their hi...

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Main Authors: Zhang, Qing, Su, Rui, Du, Wenna, Liu, Xinfeng, Zhao, Liyun, Ha, Son Tung, Xiong, Qihua
其他作者: School of Electrical and Electronic Engineering
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語言:English
出版: 2020
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spelling sg-ntu-dr.10356-1403592023-02-28T19:24:52Z Advances in small perovskite-based lasers Zhang, Qing Su, Rui Du, Wenna Liu, Xinfeng Zhao, Liyun Ha, Son Tung Xiong, Qihua School of Electrical and Electronic Engineering School of Physical and Mathematical Sciences Nanoelectronics Centre of Excellence Science::Physics Emission Lasers Lead halide perovskites have recently become a rapidly growing research field due to their great potential in next‐generation solar cells and photonic sources. As a direct bandgap semiconductor, perovskites are also promising candidates for low‐threshold and multicolor lasing devices due to their high optical gain, ease of bandgap engineering, large absorption coefficient, and low defect state density. In particular, reduced‐dimensional perovskite structures including nanoplatelets, nanowires, and quantum dots, are crucial for the development of micro‐ or nanosized laser sources for optical chips and high‐resolution imaging, etc. Here, perovskite nanophotonics, in particular the lasing properties of perovskite nanostructures, are discussed. The rapid advances of small lasers based on perovskite nanostructures using both active and passive microcavities are reviewed; these are mainly classified into four sections: thin films, nanoplatelets, nanowires, and quantum dots. Lasing performance in terms of threshold, color‐tunability, spectral coherence, and stability is introduced from both materials and microcavity respects. Fundamental photophysical mechanisms involved in the photoluminescence lasing process, from absorption, emission to gain, are discussed in order to provide insightful understanding lasing properties of different types of perovskites. Finally, some future prospects for perovskite lasing devices are provided. NRF (Natl Research Foundation, S’pore) MOE (Min. of Education, S’pore) Accepted version 2020-05-28T05:15:07Z 2020-05-28T05:15:07Z 2017 Journal Article Zhang, Q., Su, R., Du, W., Liu, X., Zhao, L., Ha, S. T., & Xiong, Q. (2017). Advances in small perovskite-based lasers. Small Methods, 1(9), 1700163-. doi:10.1002/smtd.201700163 2366-9608 https://hdl.handle.net/10356/140359 10.1002/smtd.201700163 9 1 en Small Methods This is the accepted version of the following article: Zhang, Q., Su, R., Du, W., Liu, X., Zhao, L., Ha, S. T., & Xiong, Q. (2017). Advances in small perovskite-based lasers. Small Methods, 1(9), 1700163-, which has been published in final form at https://doi.org/10.1002/smtd.201700163. This article may be used for non-commercial purposes in accordance with the Wiley Self-Archiving Policy [https://authorservices.wiley.com/authorresources/Journal-Authors/licensing/self-archiving.html]. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Emission
Lasers
spellingShingle Science::Physics
Emission
Lasers
Zhang, Qing
Su, Rui
Du, Wenna
Liu, Xinfeng
Zhao, Liyun
Ha, Son Tung
Xiong, Qihua
Advances in small perovskite-based lasers
description Lead halide perovskites have recently become a rapidly growing research field due to their great potential in next‐generation solar cells and photonic sources. As a direct bandgap semiconductor, perovskites are also promising candidates for low‐threshold and multicolor lasing devices due to their high optical gain, ease of bandgap engineering, large absorption coefficient, and low defect state density. In particular, reduced‐dimensional perovskite structures including nanoplatelets, nanowires, and quantum dots, are crucial for the development of micro‐ or nanosized laser sources for optical chips and high‐resolution imaging, etc. Here, perovskite nanophotonics, in particular the lasing properties of perovskite nanostructures, are discussed. The rapid advances of small lasers based on perovskite nanostructures using both active and passive microcavities are reviewed; these are mainly classified into four sections: thin films, nanoplatelets, nanowires, and quantum dots. Lasing performance in terms of threshold, color‐tunability, spectral coherence, and stability is introduced from both materials and microcavity respects. Fundamental photophysical mechanisms involved in the photoluminescence lasing process, from absorption, emission to gain, are discussed in order to provide insightful understanding lasing properties of different types of perovskites. Finally, some future prospects for perovskite lasing devices are provided.
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Zhang, Qing
Su, Rui
Du, Wenna
Liu, Xinfeng
Zhao, Liyun
Ha, Son Tung
Xiong, Qihua
format Article
author Zhang, Qing
Su, Rui
Du, Wenna
Liu, Xinfeng
Zhao, Liyun
Ha, Son Tung
Xiong, Qihua
author_sort Zhang, Qing
title Advances in small perovskite-based lasers
title_short Advances in small perovskite-based lasers
title_full Advances in small perovskite-based lasers
title_fullStr Advances in small perovskite-based lasers
title_full_unstemmed Advances in small perovskite-based lasers
title_sort advances in small perovskite-based lasers
publishDate 2020
url https://hdl.handle.net/10356/140359
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