Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications
Particle-assembled fluid-fluid interfaces give rise to soft substrate-less platforms with wide-ranging applications, including remote and on-demand manipulation, optical modulation, catalysis, and multiphase and multiplex sensing, as well as in situ reaction kinetics elucidation. Notably, these soft...
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sg-ntu-dr.10356-1433432023-02-28T19:25:35Z Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications Lee, Hiang Kwee Lee, Yih Hong Phan-Quang, Gia Chuong Han, Xuemei Koh, Charlynn Sher Lin Ling, Xing Yi School of Physical and Mathematical Sciences Institute of Materials Research and Engineering, A*STAR Science::Chemistry Interfaces Liquids Particle-assembled fluid-fluid interfaces give rise to soft substrate-less platforms with wide-ranging applications, including remote and on-demand manipulation, optical modulation, catalysis, and multiphase and multiplex sensing, as well as in situ reaction kinetics elucidation. Notably, these soft platforms are easy to fabricate and can exhibit long-range order, both of which are challenging to achieve using traditional solid-based substrates. In this perspective, we provide an overview of the latest research in the fabrication and applications of these soft platforms. We begin with a brief discussion on the formation mechanism of two- and three-dimensional substrate-less platforms, followed by highlighting the unique properties of these platforms. We also discuss the application of these particle-assembled interfaces to three specific research areas, including dynamic tuning of optical properties, multiplex molecular sensing, and small-volume reaction modulation and kinetics monitoring. We end our perspective with an outlook on the promising research frontiers that can be achieved using these soft substrate-less platforms. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Nanyang Technological University National Research Foundation (NRF) Accepted version X.Y.L. is grateful for the financial support from National Research Foundation, Singapore (NRF-NRFF2012-04), Singapore Ministry of Education, Tier 1 (RG21/16) and Tier 2 (MOE2016-T2-1-043) grants. H.K.L. appreciates the A*STAR Graduate Scholarship support from A*STAR, Singapore. G.C.P.-Q. and C.S.L.K acknowledge support from Nanyang Presidential Graduate Scholarship from Nanyang Technological University. 2020-08-26T02:45:39Z 2020-08-26T02:45:39Z 2017 Journal Article Lee, H. K., Lee, Y. H., Phan-Quang, G. C., Han, X., Koh, C. S. L., & Ling, X. Y. (2017). Constructing soft substrate-less platforms using particle-assembled fluid–fluid interfaces and their prospects in multiphasic applications. Chemistry of Materials, 29(16), 6563-6577. doi:10.1021/acs.chemmater.7b02227 0897-4756 https://hdl.handle.net/10356/143343 10.1021/acs.chemmater.7b02227 2-s2.0-85027979526 16 29 6563 6577 en Chemistry of Materials This document is the Accepted Manuscript version of a Published Work that appeared in final form in Chemistry of Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.chemmater.7b02227 application/pdf |
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Science::Chemistry Interfaces Liquids Lee, Hiang Kwee Lee, Yih Hong Phan-Quang, Gia Chuong Han, Xuemei Koh, Charlynn Sher Lin Ling, Xing Yi Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
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Particle-assembled fluid-fluid interfaces give rise to soft substrate-less platforms with wide-ranging applications, including remote and on-demand manipulation, optical modulation, catalysis, and multiphase and multiplex sensing, as well as in situ reaction kinetics elucidation. Notably, these soft platforms are easy to fabricate and can exhibit long-range order, both of which are challenging to achieve using traditional solid-based substrates. In this perspective, we provide an overview of the latest research in the fabrication and applications of these soft platforms. We begin with a brief discussion on the formation mechanism of two- and three-dimensional substrate-less platforms, followed by highlighting the unique properties of these platforms. We also discuss the application of these particle-assembled interfaces to three specific research areas, including dynamic tuning of optical properties, multiplex molecular sensing, and small-volume reaction modulation and kinetics monitoring. We end our perspective with an outlook on the promising research frontiers that can be achieved using these soft substrate-less platforms. |
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School of Physical and Mathematical Sciences |
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School of Physical and Mathematical Sciences Lee, Hiang Kwee Lee, Yih Hong Phan-Quang, Gia Chuong Han, Xuemei Koh, Charlynn Sher Lin Ling, Xing Yi |
format |
Article |
author |
Lee, Hiang Kwee Lee, Yih Hong Phan-Quang, Gia Chuong Han, Xuemei Koh, Charlynn Sher Lin Ling, Xing Yi |
author_sort |
Lee, Hiang Kwee |
title |
Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
title_short |
Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
title_full |
Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
title_fullStr |
Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
title_full_unstemmed |
Constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
title_sort |
constructing soft substrate-less platforms using particle-assembled fluid-fluid interfaces and their prospects in multiphasic applications |
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2020 |
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https://hdl.handle.net/10356/143343 |
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1759856134489899008 |