A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability

Traditional superhydrophobic coatings prepared from non-degradable materials tend to do harm to the environment throughout the fabrication process as well as after being discarded. Great efforts have been devoted to exploring more environmentally friendly approaches and materials to settle this prob...

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Main Authors: Dong, Xiuli, Gao, Shouwei, Huang, Jianying, Li, Shuhui, Zhu, Tianxue, Cheng, Yan, Zhao, Yan, Chen, Zhong, Lai, Yuekun
Other Authors: School of Materials Science and Engineering
Format: Article
Language:English
Published: 2020
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Online Access:https://hdl.handle.net/10356/143355
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1433552023-07-14T15:47:53Z A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability Dong, Xiuli Gao, Shouwei Huang, Jianying Li, Shuhui Zhu, Tianxue Cheng, Yan Zhao, Yan Chen, Zhong Lai, Yuekun School of Materials Science and Engineering Engineering::Materials Superhydrophobic Coatings Oil–water Separation Properties Traditional superhydrophobic coatings prepared from non-degradable materials tend to do harm to the environment throughout the fabrication process as well as after being discarded. Great efforts have been devoted to exploring more environmentally friendly approaches and materials to settle this problem. Here we report an eco-friendly strategy based on aqueous systems to construct superhydrophobic coatings on various fabrics. Fabrics were first coated with polydopamine (PDA) and then modified with the stearic acid emulsion to introduce the desired surface morphology and energy. The as-prepared fabrics achieved robust superhydrophobicity with a contact angle (CA) about 162.0° and sliding angle (SA) about 7.8°. Moreover, due to the UV-absorbing and the photo-thermal conversion ability of PDA, the modified fabrics exhibited excellent UV shielding and solar-induced self-healing properties. The as-prepared fabrics also possessed high efficiency oil–water separation properties. Without the usage of harmful organic solvents and the addition of micro/nano-particles, this biodegradable superhydrophobic fabric exhibited a clear advantage of being environmentally friendly over conventional coatings. Furthermore, the facile and low-cost fabrication process makes its large-scale production easy. Accepted version The authors thank the National Natural Science Foundation of China (21501127; 51502185), Natural Science Foundation of Jiangsu Province of China (BK20140400), and Natural Science Foundation of the Jiangsu Higher Education Institutions of China (15KJB430025). We also acknowledge the funds from the project of the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD). 2020-08-26T05:30:20Z 2020-08-26T05:30:20Z 2018 Journal Article Dong, X., Gao, S., Huang, J., Li, S., Zhu, T., Cheng, Y., ... Lai, Y. (2019). A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability. Journal of Materials Chemistry A, 7(5), 2122-2128. doi:10.1039/c8ta10869b 2050-7488 https://hdl.handle.net/10356/143355 10.1039/c8ta10869b 2-s2.0-85060825793 5 7 2122 2128 en Journal of Materials Chemistry A © 2019 The Royal Society of Chemistry. All rights reserved. This paper was published in Journal of Materials Chemistry A and is made available with permission of The Royal Society of Chemistry. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Materials
Superhydrophobic Coatings
Oil–water Separation Properties
spellingShingle Engineering::Materials
Superhydrophobic Coatings
Oil–water Separation Properties
Dong, Xiuli
Gao, Shouwei
Huang, Jianying
Li, Shuhui
Zhu, Tianxue
Cheng, Yan
Zhao, Yan
Chen, Zhong
Lai, Yuekun
A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
description Traditional superhydrophobic coatings prepared from non-degradable materials tend to do harm to the environment throughout the fabrication process as well as after being discarded. Great efforts have been devoted to exploring more environmentally friendly approaches and materials to settle this problem. Here we report an eco-friendly strategy based on aqueous systems to construct superhydrophobic coatings on various fabrics. Fabrics were first coated with polydopamine (PDA) and then modified with the stearic acid emulsion to introduce the desired surface morphology and energy. The as-prepared fabrics achieved robust superhydrophobicity with a contact angle (CA) about 162.0° and sliding angle (SA) about 7.8°. Moreover, due to the UV-absorbing and the photo-thermal conversion ability of PDA, the modified fabrics exhibited excellent UV shielding and solar-induced self-healing properties. The as-prepared fabrics also possessed high efficiency oil–water separation properties. Without the usage of harmful organic solvents and the addition of micro/nano-particles, this biodegradable superhydrophobic fabric exhibited a clear advantage of being environmentally friendly over conventional coatings. Furthermore, the facile and low-cost fabrication process makes its large-scale production easy.
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Dong, Xiuli
Gao, Shouwei
Huang, Jianying
Li, Shuhui
Zhu, Tianxue
Cheng, Yan
Zhao, Yan
Chen, Zhong
Lai, Yuekun
format Article
author Dong, Xiuli
Gao, Shouwei
Huang, Jianying
Li, Shuhui
Zhu, Tianxue
Cheng, Yan
Zhao, Yan
Chen, Zhong
Lai, Yuekun
author_sort Dong, Xiuli
title A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
title_short A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
title_full A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
title_fullStr A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
title_full_unstemmed A self-roughened and biodegradable superhydrophobic coating with UV shielding, solar-induced self-healing and versatile oil-water separation ability
title_sort self-roughened and biodegradable superhydrophobic coating with uv shielding, solar-induced self-healing and versatile oil-water separation ability
publishDate 2020
url https://hdl.handle.net/10356/143355
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