Solution processed polymer-ABX4 perovskite-like microcavities

Thanks to solution processability and broad emission in the visible spectral range, 2D hybrid perovskite-like materials are interesting for the realization of large area and flexible lighting devices. However, the deposition of these materials requires broad-spectrum solvents that can easily dissolv...

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Bibliographic Details
Main Authors: Lova, Paola, Cortecchia, Daniele, Soci, Cesare, Comoretto, Davide
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2021
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Online Access:https://hdl.handle.net/10356/146248
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Institution: Nanyang Technological University
Language: English
Description
Summary:Thanks to solution processability and broad emission in the visible spectral range, 2D hybrid perovskite-like materials are interesting for the realization of large area and flexible lighting devices. However, the deposition of these materials requires broad-spectrum solvents that can easily dissolve most of the commercial polymers and make perovskites incompatible with flexible photonics. Here, we demonstrated the integration of broadband-emitting (EDBE)PbCl4 (where EDBE = 2,2-(ethylenedioxy)bis(ethylammonium)) thin films with a solution-processed polymer planar microcavities, employing a sacrificial polymer multilayer. This approach allowed for spectral and angular redistribution of the perovskite-like material, photoluminescence, that can pave the way to all-solution-processed and flexible lightning devices that do not require complex and costly fabrication techniques.