Barrier-controlled nonequilibrium criticality in reactive particle systems

• Main Authors: Lei, Qun-Li, Hu, Hao, Ni, Ran
• Other Authors: School of Chemical and Biomedical Engineering
• Format: Article
• Language: English
• Published: 2022
• Subjects: Engineering::Chemical engineering; Molecular-Dynamics Simulation; Random Organization
• Online Access: https://hdl.handle.net/10356/154970
• Institution: Nanyang Technological University

Nonequilibrium critical phenomena generally exist in many dynamic systems, like chemical reactions and some driven-dissipative reactive particle systems. Here, by using computer simulation and theoretical analysis, we demonstrate the crucial role of the activation barrier on the criticality of dynamic phase transitions in a minimal reactive hard-sphere model. We find that at zero thermal noise, with increasing the activation barrier, the type of transition changes from a continuous conserved directed percolation into a discontinuous dynamic transition by crossing a tricritical point. A mean-field theory combined with field simulation is proposed to explain this phenomenon. The possibility of Ising-type criticality in the nonequilibrium system at finite thermal noise is also discussed.