Co-evaporated perovskite light-emitting transistor operating at room temperature

Solution-processed hybrid organic–inorganic perovskite light-emitting transistors (PeLETs) suffer from low brightness and environmental instability induced by temperature-activated trapping, ionic motion, and polarization effects, which so far have been hindering the realization of devices operating...

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Main Authors: Klein, Maciej, Li, Jia, Bruno, Annalisa, Soci, Cesare
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2022
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Online Access:https://hdl.handle.net/10356/155640
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Institution: Nanyang Technological University
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spelling sg-ntu-dr.10356-1556402022-11-04T03:26:28Z Co-evaporated perovskite light-emitting transistor operating at room temperature Klein, Maciej Li, Jia Bruno, Annalisa Soci, Cesare School of Physical and Mathematical Sciences Energy Research Institute @ NTU (ERI@N) Centre for Disruptive Photonic Technologies (CDPT) Science::Physics Methylammonium Lead Iodide Co-evaporated Perovskite Films Solution-processed hybrid organic–inorganic perovskite light-emitting transistors (PeLETs) suffer from low brightness and environmental instability induced by temperature-activated trapping, ionic motion, and polarization effects, which so far have been hindering the realization of devices operating at room temperature. Here high quality thermally co-evaporated methylammonium lead iodide perovskite films are employed to minimize ionic motion and significantly improve the electroluminescence characteristics of the perovskite active layer, enabling stable device operation up to ≈ 310 K. The demonstration of PeLETs operating at and beyond room-temperature paves the way for practical applications in the rapidly evolving area of solid-state lighting, active-matrix displays, and visible light communications. Agency for Science, Technology and Research (A*STAR) National Research Foundation (NRF) Submitted/Accepted version This research was funded by National Research Foundation, Prime Minister’s Office, Singapore under its Competitive Research Programme (CRP Award No. NRF-CRP14-2014-03; Solar CRP: S18-1176-SCRP) and by the A*STAR-AME programmatic grant on Nanoantenna Spatial Light Modulators for Next-Gen Display Technologies (Grant No. A18A7b0058). 2022-03-15T01:53:12Z 2022-03-15T01:53:12Z 2021 Journal Article Klein, M., Li, J., Bruno, A. & Soci, C. (2021). Co-evaporated perovskite light-emitting transistor operating at room temperature. Advanced Electronic Materials, 7(7), 2100403-. https://dx.doi.org/10.1002/aelm.202100403 2199-160X https://hdl.handle.net/10356/155640 10.1002/aelm.202100403 2-s2.0-85107505724 7 7 2100403 en NRF-CRP14-2014-03 S18-1176-SCRP A18A7b0058 Advanced Electronic Materials 10.21979/N9/YXYBGB This is the peer reviewed version of the following article: Klein, M., Li, J., Bruno, A. & Soci, C. (2021). Co-evaporated perovskite light-emitting transistor operating at room temperature. Advanced Electronic Materials, 7(7), 2100403-, which has been published in final form at https://doi.org/10.1002/aelm.202100403. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. application/pdf application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Methylammonium Lead Iodide
Co-evaporated Perovskite Films
spellingShingle Science::Physics
Methylammonium Lead Iodide
Co-evaporated Perovskite Films
Klein, Maciej
Li, Jia
Bruno, Annalisa
Soci, Cesare
Co-evaporated perovskite light-emitting transistor operating at room temperature
description Solution-processed hybrid organic–inorganic perovskite light-emitting transistors (PeLETs) suffer from low brightness and environmental instability induced by temperature-activated trapping, ionic motion, and polarization effects, which so far have been hindering the realization of devices operating at room temperature. Here high quality thermally co-evaporated methylammonium lead iodide perovskite films are employed to minimize ionic motion and significantly improve the electroluminescence characteristics of the perovskite active layer, enabling stable device operation up to ≈ 310 K. The demonstration of PeLETs operating at and beyond room-temperature paves the way for practical applications in the rapidly evolving area of solid-state lighting, active-matrix displays, and visible light communications.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Klein, Maciej
Li, Jia
Bruno, Annalisa
Soci, Cesare
format Article
author Klein, Maciej
Li, Jia
Bruno, Annalisa
Soci, Cesare
author_sort Klein, Maciej
title Co-evaporated perovskite light-emitting transistor operating at room temperature
title_short Co-evaporated perovskite light-emitting transistor operating at room temperature
title_full Co-evaporated perovskite light-emitting transistor operating at room temperature
title_fullStr Co-evaporated perovskite light-emitting transistor operating at room temperature
title_full_unstemmed Co-evaporated perovskite light-emitting transistor operating at room temperature
title_sort co-evaporated perovskite light-emitting transistor operating at room temperature
publishDate 2022
url https://hdl.handle.net/10356/155640
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