Hydrophobic bioadhesive composites for human motion detection

Conductive hydrogels are rapidly rising as sensing materials for bioelectronics applications, but lack mechanical and adhesion strength due to their excess water content. We propose a diazirine-grafted polycaprolactone adhesive (CaproGlu)/carbon nanotubes (CNTs) composite that can provide wet adhesi...

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Main Authors: Singh, Manisha, Solic, Ivan, Steele, Terry W. J.
Other Authors: School of Materials Science and Engineering
Format: Article
Language:English
Published: 2022
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Online Access:https://hdl.handle.net/10356/158570
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1585702023-07-14T16:04:36Z Hydrophobic bioadhesive composites for human motion detection Singh, Manisha Solic, Ivan Steele, Terry W. J. School of Materials Science and Engineering Engineering::Bioengineering Engineering::Materials::Biomaterials Bioelectronic Applications Carbon Nanotubes Composites Conductive hydrogels are rapidly rising as sensing materials for bioelectronics applications, but lack mechanical and adhesion strength due to their excess water content. We propose a diazirine-grafted polycaprolactone adhesive (CaproGlu)/carbon nanotubes (CNTs) composite that can provide wet adhesion and strong mechanical properties at the tissue-machine interface. The introduced CNTs not only reinforced the CaproGlu, but also formed electrically conducting pathways. The CaproGlu composites exhibited conductivity of 0.1 S m-1 and a charge storage capacity of 5 μC cm-2. The resulting composites are biocompatible and can be used as strain sensors to detect mechanical deformations. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Nanyang Technological University Submitted/Accepted version This work was supported by the Ministry of Education Tier 2 Grant (MOE2018-T2-2-114): CaproGlu and double-sided wet-tissue adhesives; NTUitive POC (Gap) Fund NGF/2018/ 05: Aesthetic applications of CaproGlu bioadhesives; and A*Star IAF PP Grant (H19/01/a0/0II9): CathoGlu bioadhesives-preventing catheter extravasation and skin infections. 2022-05-20T07:04:24Z 2022-05-20T07:04:24Z 2021 Journal Article Singh, M., Solic, I. & Steele, T. W. J. (2021). Hydrophobic bioadhesive composites for human motion detection. ACS Macro Letters, 10(11), 1353-1358. https://dx.doi.org/10.1021/acsmacrolett.1c00559 2161-1653 https://hdl.handle.net/10356/158570 10.1021/acsmacrolett.1c00559 35549014 2-s2.0-85118113389 11 10 1353 1358 en MOE2018-T2-2-114 NGF/2018/05 H19/01/a0/0II9 ACS Macro Letters This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Macro Letters, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acsmacrolett.1c00559. application/pdf application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Bioengineering
Engineering::Materials::Biomaterials
Bioelectronic Applications
Carbon Nanotubes Composites
spellingShingle Engineering::Bioengineering
Engineering::Materials::Biomaterials
Bioelectronic Applications
Carbon Nanotubes Composites
Singh, Manisha
Solic, Ivan
Steele, Terry W. J.
Hydrophobic bioadhesive composites for human motion detection
description Conductive hydrogels are rapidly rising as sensing materials for bioelectronics applications, but lack mechanical and adhesion strength due to their excess water content. We propose a diazirine-grafted polycaprolactone adhesive (CaproGlu)/carbon nanotubes (CNTs) composite that can provide wet adhesion and strong mechanical properties at the tissue-machine interface. The introduced CNTs not only reinforced the CaproGlu, but also formed electrically conducting pathways. The CaproGlu composites exhibited conductivity of 0.1 S m-1 and a charge storage capacity of 5 μC cm-2. The resulting composites are biocompatible and can be used as strain sensors to detect mechanical deformations.
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Singh, Manisha
Solic, Ivan
Steele, Terry W. J.
format Article
author Singh, Manisha
Solic, Ivan
Steele, Terry W. J.
author_sort Singh, Manisha
title Hydrophobic bioadhesive composites for human motion detection
title_short Hydrophobic bioadhesive composites for human motion detection
title_full Hydrophobic bioadhesive composites for human motion detection
title_fullStr Hydrophobic bioadhesive composites for human motion detection
title_full_unstemmed Hydrophobic bioadhesive composites for human motion detection
title_sort hydrophobic bioadhesive composites for human motion detection
publishDate 2022
url https://hdl.handle.net/10356/158570
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