β-In₂S₃ nanoplates for ultrafast photonics

The technological revolution of two-dimensional (2D) materials provides vitality for ultrafast optics. Compared with other 2D materials, indium sulfide (In2S3) has become an attractive candidate material in the field of nonlinear optics because of its high carrier mobility, ultrafast photoelectric s...

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Main Authors: Li, Xiaohui, Han, Yueheng, Shi, Zhaojiang, An, Mingqi, Chen, Enci, Feng, Jiangjiang, Wang, Qi Jie
Other Authors: School of Electrical and Electronic Engineering
Format: Article
Language:English
Published: 2022
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Online Access:https://hdl.handle.net/10356/161658
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1616582023-02-28T20:08:15Z β-In₂S₃ nanoplates for ultrafast photonics Li, Xiaohui Han, Yueheng Shi, Zhaojiang An, Mingqi Chen, Enci Feng, Jiangjiang Wang, Qi Jie School of Electrical and Electronic Engineering School of Physical and Mathematical Sciences Centre for OptoElectronics and Biophotonics The Photonics Institute Engineering::Electrical and electronic engineering Indium Sulfide High Repetition Rate The technological revolution of two-dimensional (2D) materials provides vitality for ultrafast optics. Compared with other 2D materials, indium sulfide (In2S3) has become an attractive candidate material in the field of nonlinear optics because of its high carrier mobility, ultrafast photoelectric sensitivity, medium band gap, and high absorption coefficient. However, its nonlinear optical effects have rarely been studied. In this work, we synthesized 2D β-In2S3nanoplates using the hydrothermal method. The saturable absorber based on β-In2S3nanoplates has been investigated. The experimental results demonstrated that the modulation depth and saturable intensity of β-In2S3are measured as 2.32% and 18.4 MW·cm-2, respectively, which indicates that β-In2S3has great potential in ultrafast optics among emerging nonlinear optical materials. Using such unprecedented properties, the mode-locked fiber laser with 247th (1.92 GHz) harmonic mode locking is realized in the C-band for the first time to our knowledge. This paves the way for exploring β-In2S3as an outstanding nonlinear material for high-performance ultrafast optics. Submitted/Accepted version This research was supported by the International Science & Technology Cooperation and Exchanges Project of Shaanxi (no. 2020KW-005); the Funded projects for the Academic Leader and Academic Backbones, Shaanxi Normal University (no. 18QNGG006); the Starting Grants of Shaanxi Normal University (grant nos. 1112010209 and 1110010717); and the Fundamental Research Funds For the Central Universities (nos. GK201802006 and 2020CSLY005). 2022-09-13T07:20:29Z 2022-09-13T07:20:29Z 2022 Journal Article Li, X., Han, Y., Shi, Z., An, M., Chen, E., Feng, J. & Wang, Q. J. (2022). β-In₂S₃ nanoplates for ultrafast photonics. ACS Applied Nano Materials, 5(3), 3229-3236. https://dx.doi.org/10.1021/acsanm.1c03542 2574-0970 https://hdl.handle.net/10356/161658 10.1021/acsanm.1c03542 2-s2.0-85127330193 3 5 3229 3236 en ACS Applied Nano Materials This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Nano Materials, copyright © 2022 American Chemical Society, after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acsanm.1c03542. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Electrical and electronic engineering
Indium Sulfide
High Repetition Rate
spellingShingle Engineering::Electrical and electronic engineering
Indium Sulfide
High Repetition Rate
Li, Xiaohui
Han, Yueheng
Shi, Zhaojiang
An, Mingqi
Chen, Enci
Feng, Jiangjiang
Wang, Qi Jie
β-In₂S₃ nanoplates for ultrafast photonics
description The technological revolution of two-dimensional (2D) materials provides vitality for ultrafast optics. Compared with other 2D materials, indium sulfide (In2S3) has become an attractive candidate material in the field of nonlinear optics because of its high carrier mobility, ultrafast photoelectric sensitivity, medium band gap, and high absorption coefficient. However, its nonlinear optical effects have rarely been studied. In this work, we synthesized 2D β-In2S3nanoplates using the hydrothermal method. The saturable absorber based on β-In2S3nanoplates has been investigated. The experimental results demonstrated that the modulation depth and saturable intensity of β-In2S3are measured as 2.32% and 18.4 MW·cm-2, respectively, which indicates that β-In2S3has great potential in ultrafast optics among emerging nonlinear optical materials. Using such unprecedented properties, the mode-locked fiber laser with 247th (1.92 GHz) harmonic mode locking is realized in the C-band for the first time to our knowledge. This paves the way for exploring β-In2S3as an outstanding nonlinear material for high-performance ultrafast optics.
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Li, Xiaohui
Han, Yueheng
Shi, Zhaojiang
An, Mingqi
Chen, Enci
Feng, Jiangjiang
Wang, Qi Jie
format Article
author Li, Xiaohui
Han, Yueheng
Shi, Zhaojiang
An, Mingqi
Chen, Enci
Feng, Jiangjiang
Wang, Qi Jie
author_sort Li, Xiaohui
title β-In₂S₃ nanoplates for ultrafast photonics
title_short β-In₂S₃ nanoplates for ultrafast photonics
title_full β-In₂S₃ nanoplates for ultrafast photonics
title_fullStr β-In₂S₃ nanoplates for ultrafast photonics
title_full_unstemmed β-In₂S₃ nanoplates for ultrafast photonics
title_sort β-in₂s₃ nanoplates for ultrafast photonics
publishDate 2022
url https://hdl.handle.net/10356/161658
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