Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties
The electrochemical hydrogen evolution reaction (HER) that converts renewable electricity into storable hydrogen, a sustainable and clean energy carrier, provides a promising method to mitigate the energy crisis and environmental pollution. In general, noble-metal-based nanomaterials (including Pt,...
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sg-ntu-dr.10356-1622692022-10-11T06:17:00Z Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties Liu, Yuhang Wang, Qilun Zhang, Jincheng Ding, Jie Cheng, Yaqi Wang, Tian Li, Jing Hu, Fangxin Yang, Hong Bin Liu, Bin School of Chemical and Biomedical Engineering Engineering::Chemical engineering Electrocatalysts Hydrogen Evolution Reaction The electrochemical hydrogen evolution reaction (HER) that converts renewable electricity into storable hydrogen, a sustainable and clean energy carrier, provides a promising method to mitigate the energy crisis and environmental pollution. In general, noble-metal-based nanomaterials (including Pt, Rh, Ru, Ir, etc.) have drawn tremendous research attention in the context of the HER because of their nearly optimal bindings to hydrogen, robust stability and tunable physical/chemical properties. Particularly, carbon as a substrate not only offers a stabilizing and conductive matrix, but also impacts the electronic structure of the supported metal by interfacial interaction, necessitating a detailed understanding. To speed up the sluggish kinetics of the HER, the design and construction of efficient electrocatalysts is of crucial importance. Herein, a comprehensive review of the recent advances in carbon-supported noble-metal electrocatalysts is presented, focusing on their synthetic strategies, structural analyses, and applications in HER electrocatalysis. Specifically, the correlation between the electronic structure and activity is discussed. Furthermore, a perspective is offered highlighting the challenges and opportunities for development of highly efficient HER electrocatalysts, with the aim for widespread utilization of practical water electrolyzers toward green hydrogen production. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) This work was financially supported by the National Natural Science Foundation of China (Grant No. 22075195), Singapore Ministry of Education Academic Research Fund (AcRF) Tier 1: RG4/20, Singapore Ministry of Education Academic Research Fund (AcRF) Tier 1: RG2/21, Singapore Ministry of Education Academic Research Fund (AcRF) Tier 2: MOET2EP10120-0002, Agency for Science, Technology and Research: AME IRG A20E5c0080, interdisciplinary project of Yangzhou University (yzuxk202013), and the starting research fund of Suzhou University of Science and Technology for H.B.Y. 2022-10-11T06:17:00Z 2022-10-11T06:17:00Z 2022 Journal Article Liu, Y., Wang, Q., Zhang, J., Ding, J., Cheng, Y., Wang, T., Li, J., Hu, F., Yang, H. B. & Liu, B. (2022). Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties. Advanced Energy Materials, 12(28), 2200928-. https://dx.doi.org/10.1002/aenm.202200928 1614-6832 https://hdl.handle.net/10356/162269 10.1002/aenm.202200928 2-s2.0-85131210250 28 12 2200928 en RG4/20 RG2/21 MOET2EP10120-0002 A20E5c0080 Advanced Energy Materials © 2022 Wiley-VCH GmbH. All rights reserved. |
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Engineering::Chemical engineering Electrocatalysts Hydrogen Evolution Reaction Liu, Yuhang Wang, Qilun Zhang, Jincheng Ding, Jie Cheng, Yaqi Wang, Tian Li, Jing Hu, Fangxin Yang, Hong Bin Liu, Bin Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
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The electrochemical hydrogen evolution reaction (HER) that converts renewable electricity into storable hydrogen, a sustainable and clean energy carrier, provides a promising method to mitigate the energy crisis and environmental pollution. In general, noble-metal-based nanomaterials (including Pt, Rh, Ru, Ir, etc.) have drawn tremendous research attention in the context of the HER because of their nearly optimal bindings to hydrogen, robust stability and tunable physical/chemical properties. Particularly, carbon as a substrate not only offers a stabilizing and conductive matrix, but also impacts the electronic structure of the supported metal by interfacial interaction, necessitating a detailed understanding. To speed up the sluggish kinetics of the HER, the design and construction of efficient electrocatalysts is of crucial importance. Herein, a comprehensive review of the recent advances in carbon-supported noble-metal electrocatalysts is presented, focusing on their synthetic strategies, structural analyses, and applications in HER electrocatalysis. Specifically, the correlation between the electronic structure and activity is discussed. Furthermore, a perspective is offered highlighting the challenges and opportunities for development of highly efficient HER electrocatalysts, with the aim for widespread utilization of practical water electrolyzers toward green hydrogen production. |
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School of Chemical and Biomedical Engineering |
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School of Chemical and Biomedical Engineering Liu, Yuhang Wang, Qilun Zhang, Jincheng Ding, Jie Cheng, Yaqi Wang, Tian Li, Jing Hu, Fangxin Yang, Hong Bin Liu, Bin |
format |
Article |
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Liu, Yuhang Wang, Qilun Zhang, Jincheng Ding, Jie Cheng, Yaqi Wang, Tian Li, Jing Hu, Fangxin Yang, Hong Bin Liu, Bin |
author_sort |
Liu, Yuhang |
title |
Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
title_short |
Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
title_full |
Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
title_fullStr |
Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
title_full_unstemmed |
Recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
title_sort |
recent advances in carbon-supported noble-metal electrocatalysts for hydrogen evolution reaction: syntheses, structures, and properties |
publishDate |
2022 |
url |
https://hdl.handle.net/10356/162269 |
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1749179203955195904 |