Microenvironment engineering for the electrocatalytic CO₂ reduction reaction
Rather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction (eCO2 RR), as previously reviewed elsewhere, we herein extend the discussion to the special topic of the microenvironment around the electrocatalytic center and present a comprehensive overview of recent...
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sg-ntu-dr.10356-1634692022-12-07T04:25:47Z Microenvironment engineering for the electrocatalytic CO₂ reduction reaction Lv, Jing-Jing Yin, Ruonan Zhou, Limin Li, Jun Kikas, Reddu Xu, Ting Wang, Zheng-Jun Jin, Huile Wang, Xin Wang, Shun School of Chemical and Biomedical Engineering Engineering::Chemical engineering Reduction Reaction Microenvironment Engineering Rather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction (eCO2 RR), as previously reviewed elsewhere, we herein extend the discussion to the special topic of the microenvironment around the electrocatalytic center and present a comprehensive overview of recent research progress. We categorize the microenvironment based on the components relevant to electrocatalytic active sites, i.e., the catalyst surface, substrate, co-reactants, electrolyte, membrane, and reactor. Supported by most of the reported articles, the relevant factors affecting the catalytic performance of eCO2 RR are then discussed in detail, and existing challenges and potential solutions are mentioned. Perspectives for the future research on eCO2 RR, including the integration of different microenvironment factors, the extension to industrial application by coupling with carbon capture and conversion, and separation of products, are also discussed. This work was financially supported by the National Natural Science Foundation of China (51872209, 52072273), Zhejiang Provincial Special Support Program for High-level Talents (2019R52042), and Wenzhou basic scientific research project (No.2020G0076). J. J. Lv would like to acknowledge the Start-up Fund of Wenzhou University (QD2021152). 2022-12-07T04:25:47Z 2022-12-07T04:25:47Z 2022 Journal Article Lv, J., Yin, R., Zhou, L., Li, J., Kikas, R., Xu, T., Wang, Z., Jin, H., Wang, X. & Wang, S. (2022). Microenvironment engineering for the electrocatalytic CO₂ reduction reaction. Angewandte Chemie (International Ed. in English), 61(39), e202207252-. https://dx.doi.org/10.1002/anie.202207252 1433-7851 https://hdl.handle.net/10356/163469 10.1002/anie.202207252 35819244 2-s2.0-85136660366 39 61 e202207252 en Angewandte Chemie (International ed. in English) © 2022 Wiley-VCH GmbH. All rights reserved. |
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Engineering::Chemical engineering Reduction Reaction Microenvironment Engineering Lv, Jing-Jing Yin, Ruonan Zhou, Limin Li, Jun Kikas, Reddu Xu, Ting Wang, Zheng-Jun Jin, Huile Wang, Xin Wang, Shun Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
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Rather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction (eCO2 RR), as previously reviewed elsewhere, we herein extend the discussion to the special topic of the microenvironment around the electrocatalytic center and present a comprehensive overview of recent research progress. We categorize the microenvironment based on the components relevant to electrocatalytic active sites, i.e., the catalyst surface, substrate, co-reactants, electrolyte, membrane, and reactor. Supported by most of the reported articles, the relevant factors affecting the catalytic performance of eCO2 RR are then discussed in detail, and existing challenges and potential solutions are mentioned. Perspectives for the future research on eCO2 RR, including the integration of different microenvironment factors, the extension to industrial application by coupling with carbon capture and conversion, and separation of products, are also discussed. |
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School of Chemical and Biomedical Engineering |
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School of Chemical and Biomedical Engineering Lv, Jing-Jing Yin, Ruonan Zhou, Limin Li, Jun Kikas, Reddu Xu, Ting Wang, Zheng-Jun Jin, Huile Wang, Xin Wang, Shun |
format |
Article |
author |
Lv, Jing-Jing Yin, Ruonan Zhou, Limin Li, Jun Kikas, Reddu Xu, Ting Wang, Zheng-Jun Jin, Huile Wang, Xin Wang, Shun |
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Lv, Jing-Jing |
title |
Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
title_short |
Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
title_full |
Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
title_fullStr |
Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
title_full_unstemmed |
Microenvironment engineering for the electrocatalytic CO₂ reduction reaction |
title_sort |
microenvironment engineering for the electrocatalytic co₂ reduction reaction |
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2022 |
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https://hdl.handle.net/10356/163469 |
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1753801173057404928 |