A two-dimensional van der Waals heterostructure with isolated electron-deficient cobalt sites toward high-efficiency co2 electroreduction

• Main Authors: Gu, Huoliang, Shi, Guoshuai, Zhong, Lixiang, Liu, Lingmei, Zhang, Honghao, Yang, Chunlei, Yu, Ke, Zhu, Chenyuan, Li, Jiong, Zhang, Shuo, Chen, Chen, Han, Yu, Li, Shuzhou, Zhang, Liming
• Other Authors: School of Materials Science and Engineering
• Format: Article
• Language: English
• Published: 2022
• Subjects: Engineering::Materials; Metal-Organic Frameworks; Carbon-Dioxide
• Online Access: https://hdl.handle.net/10356/163720
• Institution: Nanyang Technological University

Electrochemical CO2 conversion is a promising way for sustainable chemical fuel production, yet the conversion efficiency is strongly limited by the sluggish kinetics and complex reaction pathways. Here we report the ultrathin conjugated metalloporphyrin covalent organic framework epitaxially grown...