Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution

Flexural oscillations of freestanding films, nanomembranes, and nanowires are attracting growing attention for their importance to the fundamental physical and optical properties and device applications of two-dimensional and nanostructured (meta)materials. Here, we report on the observation of shor...

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Main Authors: Liu, Tongjun, Ou, Jun-Yu, Papasimakis, Nikitas, MacDonald, Kevin F., Gusev, Vitalyi E., Zheludev, Nikolay I.
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/164372
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1643722023-02-28T20:10:16Z Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution Liu, Tongjun Ou, Jun-Yu Papasimakis, Nikitas MacDonald, Kevin F. Gusev, Vitalyi E. Zheludev, Nikolay I. School of Physical and Mathematical Sciences Centre for Disruptive Photonic Technologies (CDPT) The Photonics Institute Science::Physics Flexural Modes Freestanding Films Flexural oscillations of freestanding films, nanomembranes, and nanowires are attracting growing attention for their importance to the fundamental physical and optical properties and device applications of two-dimensional and nanostructured (meta)materials. Here, we report on the observation of short-time scale ballistic motion in the flexural mode of a nanomembrane cantilever, driven by thermal fluctuation of flexural phonons, including measurements of ballistic velocities and displacements performed with subatomic resolution, using a free electron edge-scattering technique. Within intervals <10 μs, the membrane moves ballistically at a constant velocity, typically ~300 μm/s, while Brownian-like dynamics emerge for longer observation periods. Access to the ballistic regime provides verification of the equipartition theorem and Maxwell-Boltzmann statistics for flexural modes and can be used in fast thermometry and mass sensing during atomic absorption/desorption processes on the membrane. Ministry of Education (MOE) Published version This work was supported by the Engineering and Physical Sciences Research Council, UK— EP/M009122/1 and EP/T02643X/1 (to N.I.Z., K.F.M., and J.-Y.O.); the Ministry of Education, Singapore—MOE2016-T3-1-006 (to N.I.Z.); and the China Scholarship Council—201806160012 (to T.L.). 2023-01-18T02:31:03Z 2023-01-18T02:31:03Z 2022 Journal Article Liu, T., Ou, J., Papasimakis, N., MacDonald, K. F., Gusev, V. E. & Zheludev, N. I. (2022). Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution. Science Advances, 8(33), eabn8007-. https://dx.doi.org/10.1126/sciadv.abn8007 2375-2548 https://hdl.handle.net/10356/164372 10.1126/sciadv.abn8007 35984884 2-s2.0-85136200331 33 8 eabn8007 en MOE2016-T3-1-006 Science Advances © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Flexural Modes
Freestanding Films
spellingShingle Science::Physics
Flexural Modes
Freestanding Films
Liu, Tongjun
Ou, Jun-Yu
Papasimakis, Nikitas
MacDonald, Kevin F.
Gusev, Vitalyi E.
Zheludev, Nikolay I.
Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
description Flexural oscillations of freestanding films, nanomembranes, and nanowires are attracting growing attention for their importance to the fundamental physical and optical properties and device applications of two-dimensional and nanostructured (meta)materials. Here, we report on the observation of short-time scale ballistic motion in the flexural mode of a nanomembrane cantilever, driven by thermal fluctuation of flexural phonons, including measurements of ballistic velocities and displacements performed with subatomic resolution, using a free electron edge-scattering technique. Within intervals <10 μs, the membrane moves ballistically at a constant velocity, typically ~300 μm/s, while Brownian-like dynamics emerge for longer observation periods. Access to the ballistic regime provides verification of the equipartition theorem and Maxwell-Boltzmann statistics for flexural modes and can be used in fast thermometry and mass sensing during atomic absorption/desorption processes on the membrane.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Liu, Tongjun
Ou, Jun-Yu
Papasimakis, Nikitas
MacDonald, Kevin F.
Gusev, Vitalyi E.
Zheludev, Nikolay I.
format Article
author Liu, Tongjun
Ou, Jun-Yu
Papasimakis, Nikitas
MacDonald, Kevin F.
Gusev, Vitalyi E.
Zheludev, Nikolay I.
author_sort Liu, Tongjun
title Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
title_short Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
title_full Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
title_fullStr Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
title_full_unstemmed Ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
title_sort ballistic dynamics of flexural thermal movements in a nanomembrane revealed with subatomic resolution
publishDate 2023
url https://hdl.handle.net/10356/164372
_version_ 1759857146553434112