Magnetically tunable spontaneous superradiance from mesoscopic perovskite emitter clusters
Perovskite emitters are promising materials as next-generation optical sources due to their low fabrication cost and high quantum yield. In particular, the superradiant emission from a few coherently coupled perovskite emitters can be used to produce a bright entangled photon source. Here, we report...
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| Main Authors: | , , , , , , , , |
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| Other Authors: | |
| Format: | Article |
| Language: | English |
| Published: |
2023
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| Subjects: | |
| Online Access: | https://hdl.handle.net/10356/168943 |
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| Institution: | Nanyang Technological University |
| Language: | English |
| Summary: | Perovskite emitters are promising materials as next-generation optical sources due to their low fabrication cost and high quantum yield. In particular, the superradiant emission from a few coherently coupled perovskite emitters can be used to produce a bright entangled photon source. Here, we report the observation of superradiance from mesoscopic (<55) CsPbBr3 perovskite emitters, which have a much smaller ensemble size than the previously reported results (>106 emitters). The superradiance is spontaneously generated by off-resonance excitation and detected by time-resolved photoluminescence and second-order photon correlation measurements. We observed a remarkable magnetic tunability of the superradiant photon bunching, indicating a magnetic field-induced decoherence process. The experimental results can be well explained using a theoretical framework based on the microscopic master equation. Our findings shed light on the superradiance mechanism in perovskite emitters and enable low-cost quantum light sources based on perovskite. |
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