Smith–Purcell radiation from highly mobile carriers in 2D quantum materials

Terahertz (THz) radiation has broad applications ranging from medical imaging to spectroscopy due to its useful properties, such as strong absorption by organic materials. One viable source of high-intensity THz radiation is the Smith-Purcell (SP) effect, which 1 involves charge carriers moving ove...

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Main Authors: Lu, Shengyuan, Nussupbekov, Ayan, Xiong, Xiao, Ding, Wen Jun, Png, Ching Eng, Ooi, Zi En, Teng, Jing Hua, Wong, Liang Jie, Chong, Yidong, Wu, Lin
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/169220
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Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-169220
record_format dspace
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics::Radiation physics
Terahertz Radiation
2D Materials
spellingShingle Science::Physics::Radiation physics
Terahertz Radiation
2D Materials
Lu, Shengyuan
Nussupbekov, Ayan
Xiong, Xiao
Ding, Wen Jun
Png, Ching Eng
Ooi, Zi En
Teng, Jing Hua
Wong, Liang Jie
Chong, Yidong
Wu, Lin
Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
description Terahertz (THz) radiation has broad applications ranging from medical imaging to spectroscopy due to its useful properties, such as strong absorption by organic materials. One viable source of high-intensity THz radiation is the Smith-Purcell (SP) effect, which 1 involves charge carriers moving over a periodic surface. Conventional SP emitters use electron beams to generate charge carriers, necessitating bulky electron acceleration stages. Here, we propose a compact design for generating THz SP radiation using mobile charge carriers within 2D materials. This circumvents the beam alignment and beam divergence challenge, allowing for a reduction in the electron-grating separation from tens of nm to 5 nm or less, leading to more efficient near-field excitation and a potentially chip-level THz source. In such a configuration, we show that the optimal electron velocity and the corresponding maximum radiation intensity can be predicted from the electron-grating separation. For graphene on a silicon grating, we numerically demonstrate how SP radiation is excited by hot electrons, including how the radiation intensity can be enhanced by graphene surface plasmons and modified by tuning the Fermi level in the graphene sheet. Due to the high carrier concentration in graphene, the radiation intensity may be further enhanced through coherent interference. This study can be extended to a broad variety of charge carriers in 2D materials, including electrons, holes, and trions, mobilized through various means such as photoexcitation and external electric fields. Utilizing intrinsic mobile carriers in 2D materials may thus allow for compact, tunable, and low-cost THz sources.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Lu, Shengyuan
Nussupbekov, Ayan
Xiong, Xiao
Ding, Wen Jun
Png, Ching Eng
Ooi, Zi En
Teng, Jing Hua
Wong, Liang Jie
Chong, Yidong
Wu, Lin
format Article
author Lu, Shengyuan
Nussupbekov, Ayan
Xiong, Xiao
Ding, Wen Jun
Png, Ching Eng
Ooi, Zi En
Teng, Jing Hua
Wong, Liang Jie
Chong, Yidong
Wu, Lin
author_sort Lu, Shengyuan
title Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
title_short Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
title_full Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
title_fullStr Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
title_full_unstemmed Smith–Purcell radiation from highly mobile carriers in 2D quantum materials
title_sort smith–purcell radiation from highly mobile carriers in 2d quantum materials
publishDate 2023
url https://hdl.handle.net/10356/169220
_version_ 1772826688062750720
spelling sg-ntu-dr.10356-1692202023-07-10T15:34:30Z Smith–Purcell radiation from highly mobile carriers in 2D quantum materials Lu, Shengyuan Nussupbekov, Ayan Xiong, Xiao Ding, Wen Jun Png, Ching Eng Ooi, Zi En Teng, Jing Hua Wong, Liang Jie Chong, Yidong Wu, Lin School of Physical and Mathematical Sciences School of Electrical and Electronic Engineering Institute of High Performance Computing, A*STAR Science::Physics::Radiation physics Terahertz Radiation 2D Materials Terahertz (THz) radiation has broad applications ranging from medical imaging to spectroscopy due to its useful properties, such as strong absorption by organic materials. One viable source of high-intensity THz radiation is the Smith-Purcell (SP) effect, which 1 involves charge carriers moving over a periodic surface. Conventional SP emitters use electron beams to generate charge carriers, necessitating bulky electron acceleration stages. Here, we propose a compact design for generating THz SP radiation using mobile charge carriers within 2D materials. This circumvents the beam alignment and beam divergence challenge, allowing for a reduction in the electron-grating separation from tens of nm to 5 nm or less, leading to more efficient near-field excitation and a potentially chip-level THz source. In such a configuration, we show that the optimal electron velocity and the corresponding maximum radiation intensity can be predicted from the electron-grating separation. For graphene on a silicon grating, we numerically demonstrate how SP radiation is excited by hot electrons, including how the radiation intensity can be enhanced by graphene surface plasmons and modified by tuning the Fermi level in the graphene sheet. Due to the high carrier concentration in graphene, the radiation intensity may be further enhanced through coherent interference. This study can be extended to a broad variety of charge carriers in 2D materials, including electrons, holes, and trions, mobilized through various means such as photoexcitation and external electric fields. Utilizing intrinsic mobile carriers in 2D materials may thus allow for compact, tunable, and low-cost THz sources. Agency for Science, Technology and Research (A*STAR) National Research Foundation (NRF) Submitted/Accepted version This work was supported by the National Research Foundation Singapore via Grant No. NRF-CRP26-2021-0004. L.W. gratefully acknowledges the Singapore University of Technology and Design for the Start-Up Research Grant SRG SMT 2021169 and Kickstarter Initiative (SKI) SKI 2021-02-14, and the National Re-search Foundation Singapore via Grant No. NRF2021-QEP2-02-P03 and NRF2021-QEP2-03-P09. S.L. acknowledges the A∗STAR National Science Scholarship. W.J.D acknowledges the support of the National Research Foundation Singapore via Grant No. NRF-CRP17-2017-08. L.J.W. acknowledges the support of the National Research Foundation Singapore Grant No. NRF2020-NRF-ISF004-3525. J.H.T. acknowledges the support of the Agency for Science, Technology and Research (A*STAR) AME IRG GrantA20E5c0084. 2023-07-10T05:37:21Z 2023-07-10T05:37:21Z 2023 Journal Article Lu, S., Nussupbekov, A., Xiong, X., Ding, W. J., Png, C. E., Ooi, Z. E., Teng, J. H., Wong, L. J., Chong, Y. & Wu, L. (2023). Smith–Purcell radiation from highly mobile carriers in 2D quantum materials. Laser & Photonics Reviews, 17(7), 2300002-. https://dx.doi.org/10.1002/lpor.202300002 1863-8880 https://hdl.handle.net/10356/169220 10.1002/lpor.202300002 7 17 2300002 en NRF- CRP26-2021-0004 SRG SMT 2021 169 SKI 2021-02-14 NRF2021-QEP2-02-P03 NRF2021-QEP2-03-P09 NRF-CRP17-2017-08 NRF2020-NRF-ISF004-3525 Laser & Photonics Reviews © 2023 Wiley-VCH GmbH. All rights reserved. This is the peer reviewed version of the following article: Lu, S., Nussupbekov, A., Xiong, X., Ding, W. J., Png, C. E., Ooi, Z. E., Teng, J. H., Wong, L. J., Chong, Y. & Wu, L. (2023). Smith–Purcell radiation from highly mobile carriers in 2D quantum materials. Laser & Photonics Reviews, 17(7), 2300002-, which has been published in final form at https://doi.org/10.1002/lpor.202300002. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. application/pdf