Tunable metasurfaces for active nanophotonics

The ability to control light propagation is a central key in optics. Conventional optical components rely on the concept of light diffraction and the gradual accumulation of the light phase as it propagates through the optical medium. However, the accumulated light phase is limited by the material t...

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Main Author: Omar Abdelrahman Mohamed Abdelraouf
Other Authors: Wang Qijie
Format: Thesis-Doctor of Philosophy
Language:English
Published: Nanyang Technological University 2023
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Online Access:https://hdl.handle.net/10356/169814
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Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-169814
record_format dspace
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Physics
spellingShingle Physics
Omar Abdelrahman Mohamed Abdelraouf
Tunable metasurfaces for active nanophotonics
description The ability to control light propagation is a central key in optics. Conventional optical components rely on the concept of light diffraction and the gradual accumulation of the light phase as it propagates through the optical medium. However, the accumulated light phase is limited by the material thickness and its permittivity. Such a mechanism often results in very bulky optical components thicker than the operating light wavelength. Recently, metasurfaces have attracted significant attention owing to their possibility to manipulate the incident light properties such as amplitude, polarization, phase, and wavefront. Metasurfaces consist of small unit cells called meta-atoms, where each meta-atom can impose different light scattering properties based on its dimensions or orientations. As a result, metasurfaces have generalized the light diffraction law by precisely designing the optical response of each meta-atom inside metasurfaces, an abrupt light phase change is achieved and changes properties of transmitted, reflected, and absorbed light. This advantage of metasurfaces enables the shrinking of many bulky optical components into a thin layer of artificially engineered nanostructures. Since the optical response of metasurfaces depends on the dimensions, optical properties, and orientations of meta-atoms, achieving reconfigurability in metasurface performance will require tuning the optical properties or dimensions of these meta-atoms. Dynamic control of metasurface behavior is favorable to tune the novel optical performance of the passive metasurface or to achieve multi-functional optical devices as an ultimate goal. Tunable materials enable dynamic control of their optical properties by using external stimuli such as electrical, optical, thermal, chemical, magnetic, and elastic strain, to name a few. Integration of tunable materials inside passive metasurfaces results in the emergent field of tunable metasurfaces. In this thesis, we present our efforts toward achieving tunable metasurfaces to empower nanophotonics devices. We introduce a paradigm of tunable metasurfaces for dynamic performance of the electromagnetic waves for applications in nonlinear optics and light emission devices. By investigating the optical and thermal modulation mechanism to tune optical properties of phase change materials (PCMs) and designing tunable metasurface incorporating PCMs to tune the meta-atom response. We were able to design and experimentally demonstrate tunable third-harmonic generation (THG) in the visible spectrum based on amorphous silicon (a-Si) metasurface supporting Fano resonance. In addition, we experimentally showed tunable light sources based on the amplified spontaneous emission concept in visible and near-infrared regimes by designing two different tunable metasurfaces that support the bound states in the continuum resonance. Moreover, many thin-film structural colors have been demonstrated using the concept of intermediate states in PCMs. Lastly, we showed an all-optical fast reconfigurable phase tuning mechanism for a fast dynamic response. The ability to individually control the optical response of each meta-atoms has made tunable metasurface to be progressively ubiquitous by enabling a wide range of novel optical functionalities. The future prospect of the conducted research work can be done by incorporating atomically thin materials (2D materials) that support ultrafast carrier dynamics and large optical properties contrast for dynamic quantum optics applications such as tunable single-photon emitters and on-chip photonic systems like a neuromorphic chip.
author2 Wang Qijie
author_facet Wang Qijie
Omar Abdelrahman Mohamed Abdelraouf
format Thesis-Doctor of Philosophy
author Omar Abdelrahman Mohamed Abdelraouf
author_sort Omar Abdelrahman Mohamed Abdelraouf
title Tunable metasurfaces for active nanophotonics
title_short Tunable metasurfaces for active nanophotonics
title_full Tunable metasurfaces for active nanophotonics
title_fullStr Tunable metasurfaces for active nanophotonics
title_full_unstemmed Tunable metasurfaces for active nanophotonics
title_sort tunable metasurfaces for active nanophotonics
publisher Nanyang Technological University
publishDate 2023
url https://hdl.handle.net/10356/169814
_version_ 1814047145667330048
spelling sg-ntu-dr.10356-1698142024-07-31T07:03:01Z Tunable metasurfaces for active nanophotonics Omar Abdelrahman Mohamed Abdelraouf Wang Qijie Wang Xiao, Renshaw School of Physical and Mathematical Sciences A*STAR Institute of Material Research and Engineering renshaw@ntu.edu.sg, qjwang@ntu.edu.sg Physics The ability to control light propagation is a central key in optics. Conventional optical components rely on the concept of light diffraction and the gradual accumulation of the light phase as it propagates through the optical medium. However, the accumulated light phase is limited by the material thickness and its permittivity. Such a mechanism often results in very bulky optical components thicker than the operating light wavelength. Recently, metasurfaces have attracted significant attention owing to their possibility to manipulate the incident light properties such as amplitude, polarization, phase, and wavefront. Metasurfaces consist of small unit cells called meta-atoms, where each meta-atom can impose different light scattering properties based on its dimensions or orientations. As a result, metasurfaces have generalized the light diffraction law by precisely designing the optical response of each meta-atom inside metasurfaces, an abrupt light phase change is achieved and changes properties of transmitted, reflected, and absorbed light. This advantage of metasurfaces enables the shrinking of many bulky optical components into a thin layer of artificially engineered nanostructures. Since the optical response of metasurfaces depends on the dimensions, optical properties, and orientations of meta-atoms, achieving reconfigurability in metasurface performance will require tuning the optical properties or dimensions of these meta-atoms. Dynamic control of metasurface behavior is favorable to tune the novel optical performance of the passive metasurface or to achieve multi-functional optical devices as an ultimate goal. Tunable materials enable dynamic control of their optical properties by using external stimuli such as electrical, optical, thermal, chemical, magnetic, and elastic strain, to name a few. Integration of tunable materials inside passive metasurfaces results in the emergent field of tunable metasurfaces. In this thesis, we present our efforts toward achieving tunable metasurfaces to empower nanophotonics devices. We introduce a paradigm of tunable metasurfaces for dynamic performance of the electromagnetic waves for applications in nonlinear optics and light emission devices. By investigating the optical and thermal modulation mechanism to tune optical properties of phase change materials (PCMs) and designing tunable metasurface incorporating PCMs to tune the meta-atom response. We were able to design and experimentally demonstrate tunable third-harmonic generation (THG) in the visible spectrum based on amorphous silicon (a-Si) metasurface supporting Fano resonance. In addition, we experimentally showed tunable light sources based on the amplified spontaneous emission concept in visible and near-infrared regimes by designing two different tunable metasurfaces that support the bound states in the continuum resonance. Moreover, many thin-film structural colors have been demonstrated using the concept of intermediate states in PCMs. Lastly, we showed an all-optical fast reconfigurable phase tuning mechanism for a fast dynamic response. The ability to individually control the optical response of each meta-atoms has made tunable metasurface to be progressively ubiquitous by enabling a wide range of novel optical functionalities. The future prospect of the conducted research work can be done by incorporating atomically thin materials (2D materials) that support ultrafast carrier dynamics and large optical properties contrast for dynamic quantum optics applications such as tunable single-photon emitters and on-chip photonic systems like a neuromorphic chip. Doctor of Philosophy 2023-08-07T05:47:12Z 2023-08-07T05:47:12Z 2023 Thesis-Doctor of Philosophy Omar Abdelrahman Mohamed Abdelraouf (2023). Tunable metasurfaces for active nanophotonics. Doctoral thesis, Nanyang Technological University, Singapore. https://hdl.handle.net/10356/169814 https://hdl.handle.net/10356/169814 10.32657/10356/169814 en 10.1002/adfm.202104627 10.1021/acsnano.2c04628 This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License (CC BY-NC 4.0). application/pdf Nanyang Technological University