Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄
We report the utilization of single-molecule fluorescence microscopy to in situ quantify the photo-oxidation reaction kinetics on g-C3N4. The wrinkle structure shows the highest reactivity and direct dissociation rate. The basal plane exhibits the highest affinity to reactants and products and indir...
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sg-ntu-dr.10356-1701962023-08-31T03:20:28Z Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ Wu, Shuyang Madridejos, Jenica Marie L. Lee, Jinn-Kye Xu, Rong Lu, Yunpeng Zhang, Zhengyang School of Chemistry, Chemical Engineering and Biotechnology Engineering::Chemical engineering Dissociation Fluorescence Microscopy We report the utilization of single-molecule fluorescence microscopy to in situ quantify the photo-oxidation reaction kinetics on g-C3N4. The wrinkle structure shows the highest reactivity and direct dissociation rate. The basal plane exhibits the highest affinity to reactants and products and indirect dissociation rate constant, followed by edges and wrinkles. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) We acknowledge the financial support from the Ministry of Education, Singapore, under its Academic Research Fund Tier 1 (No. RG10/20, RG60/21 and RG83/20), and the Singapore Agency for Science, Technology and Research (A*STAR) AME YIRG grant (No. A2084c0065) and MTC IRG grant (No. M21K2c0110). 2023-08-31T03:20:27Z 2023-08-31T03:20:27Z 2023 Journal Article Wu, S., Madridejos, J. M. L., Lee, J., Xu, R., Lu, Y. & Zhang, Z. (2023). Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄. Chemical Communications, 59(26), 3918-3921. https://dx.doi.org/10.1039/D3CC00750B 1359-7345 https://hdl.handle.net/10356/170196 10.1039/D3CC00750B 26 59 3918 3921 en RG10/20 RG60/21 RG83/20 A2084c0065 M21K2c0110 Chemical Communications © 2023 The Royal Society of Chemistry. All rights reserved. |
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Engineering::Chemical engineering Dissociation Fluorescence Microscopy Wu, Shuyang Madridejos, Jenica Marie L. Lee, Jinn-Kye Xu, Rong Lu, Yunpeng Zhang, Zhengyang Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| description |
We report the utilization of single-molecule fluorescence microscopy to in situ quantify the photo-oxidation reaction kinetics on g-C3N4. The wrinkle structure shows the highest reactivity and direct dissociation rate. The basal plane exhibits the highest affinity to reactants and products and indirect dissociation rate constant, followed by edges and wrinkles. |
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School of Chemistry, Chemical Engineering and Biotechnology |
| author_facet |
School of Chemistry, Chemical Engineering and Biotechnology Wu, Shuyang Madridejos, Jenica Marie L. Lee, Jinn-Kye Xu, Rong Lu, Yunpeng Zhang, Zhengyang |
| format |
Article |
| author |
Wu, Shuyang Madridejos, Jenica Marie L. Lee, Jinn-Kye Xu, Rong Lu, Yunpeng Zhang, Zhengyang |
| author_sort |
Wu, Shuyang |
| title |
Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| title_short |
Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| title_full |
Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| title_fullStr |
Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| title_full_unstemmed |
Quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2D g-C₃N₄ |
| title_sort |
quantitative single-molecule study reveals site-specific photo-oxidation activities and kinetics on 2d g-c₃n₄ |
| publishDate |
2023 |
| url |
https://hdl.handle.net/10356/170196 |
| _version_ |
1779156768811646976 |