Spin defects in hBN assisted by metallic nanotrenches for quantum sensing

The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as...

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Main Authors: Cai, Hongbing, Ru, Shihao, Jiang, Zhengzhi, Eng, John Jun Hong, He, Ruihua, Li, Fuli, Miao, Yansong, Zúñiga-Pérez, Jesús, Gao, Weibo
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/171095
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1710952023-10-16T15:36:22Z Spin defects in hBN assisted by metallic nanotrenches for quantum sensing Cai, Hongbing Ru, Shihao Jiang, Zhengzhi Eng, John Jun Hong He, Ruihua Li, Fuli Miao, Yansong Zúñiga-Pérez, Jesús Gao, Weibo School of Physical and Mathematical Sciences School of Biological Sciences Institute of Materials Research and Engineering, A*STAR Centre for Disruptive Photonic Technologies (CDPT) The Photonics Institute Science::Physics Hexagonal Boron Nitride Tunable Plasmonic The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as it can be easily generated while its spin population can be initialized and read out by optical means at room-temperature. But the lower quantum yield hinders its widespread use as an integrated quantum sensor. Here, we demonstrate an emission enhancement amounting to 400 by nanotrench arrays compatible with coplanar waveguide (CPW) electrodes employed for spin-state detection. By monitoring the reflectance spectrum of the resonators as additional layers of hBN are transferred, we have optimized the overall hBN/nanotrench optical response, maximizing thereby the luminescence enhancement. Based on these finely tuned heterostructures, we achieved an enhanced DC magnetic field sensitivity as high as 6 × 10-5 T/Hz1/2. Agency for Science, Technology and Research (A*STAR) National Research Foundation (NRF) Submitted/Accepted version This research is supported by the National Research Foundsation, Singapore, and A*STAR under its Quantum Engineering Programme (No. NRF2021-QEP2-03-P09, NRF2021-QEP2-01-P02, NRF2021-QEP2-01-P01, NRF2021-QEP2-03-P01, No. NRF2021-QEP2-03-P10, NRF2022-QEP2-02-P13) and IRG programme (M21K2c0116). 2023-10-13T00:52:53Z 2023-10-13T00:52:53Z 2023 Journal Article Cai, H., Ru, S., Jiang, Z., Eng, J. J. H., He, R., Li, F., Miao, Y., Zúñiga-Pérez, J. & Gao, W. (2023). Spin defects in hBN assisted by metallic nanotrenches for quantum sensing. Nano Letters, 23(11), 4991-4996. https://dx.doi.org/10.1021/acs.nanolett.3c00849 1530-6984 https://hdl.handle.net/10356/171095 10.1021/acs.nanolett.3c00849 37205843 2-s2.0-85162833679 11 23 4991 4996 en NRF2021-QEP2-03-P09 NRF2021-QEP2-01-P02 NRF2021-QEP2-01-P01 NRF2021-QEP2-03-P01 NRF2021-QEP2-03-P10 NRF2022-QEP2-02-P13 M21K2c0116 Nano Letters © 2023 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acs.nanolett.3c00849. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Hexagonal Boron Nitride
Tunable Plasmonic
spellingShingle Science::Physics
Hexagonal Boron Nitride
Tunable Plasmonic
Cai, Hongbing
Ru, Shihao
Jiang, Zhengzhi
Eng, John Jun Hong
He, Ruihua
Li, Fuli
Miao, Yansong
Zúñiga-Pérez, Jesús
Gao, Weibo
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
description The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as it can be easily generated while its spin population can be initialized and read out by optical means at room-temperature. But the lower quantum yield hinders its widespread use as an integrated quantum sensor. Here, we demonstrate an emission enhancement amounting to 400 by nanotrench arrays compatible with coplanar waveguide (CPW) electrodes employed for spin-state detection. By monitoring the reflectance spectrum of the resonators as additional layers of hBN are transferred, we have optimized the overall hBN/nanotrench optical response, maximizing thereby the luminescence enhancement. Based on these finely tuned heterostructures, we achieved an enhanced DC magnetic field sensitivity as high as 6 × 10-5 T/Hz1/2.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Cai, Hongbing
Ru, Shihao
Jiang, Zhengzhi
Eng, John Jun Hong
He, Ruihua
Li, Fuli
Miao, Yansong
Zúñiga-Pérez, Jesús
Gao, Weibo
format Article
author Cai, Hongbing
Ru, Shihao
Jiang, Zhengzhi
Eng, John Jun Hong
He, Ruihua
Li, Fuli
Miao, Yansong
Zúñiga-Pérez, Jesús
Gao, Weibo
author_sort Cai, Hongbing
title Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
title_short Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
title_full Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
title_fullStr Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
title_full_unstemmed Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
title_sort spin defects in hbn assisted by metallic nanotrenches for quantum sensing
publishDate 2023
url https://hdl.handle.net/10356/171095
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