Spin defects in hBN assisted by metallic nanotrenches for quantum sensing
The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as...
Saved in:
Main Authors: | , , , , , , , , |
---|---|
Other Authors: | |
Format: | Article |
Language: | English |
Published: |
2023
|
Subjects: | |
Online Access: | https://hdl.handle.net/10356/171095 |
Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
Institution: | Nanyang Technological University |
Language: | English |
id |
sg-ntu-dr.10356-171095 |
---|---|
record_format |
dspace |
spelling |
sg-ntu-dr.10356-1710952023-10-16T15:36:22Z Spin defects in hBN assisted by metallic nanotrenches for quantum sensing Cai, Hongbing Ru, Shihao Jiang, Zhengzhi Eng, John Jun Hong He, Ruihua Li, Fuli Miao, Yansong Zúñiga-Pérez, Jesús Gao, Weibo School of Physical and Mathematical Sciences School of Biological Sciences Institute of Materials Research and Engineering, A*STAR Centre for Disruptive Photonic Technologies (CDPT) The Photonics Institute Science::Physics Hexagonal Boron Nitride Tunable Plasmonic The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as it can be easily generated while its spin population can be initialized and read out by optical means at room-temperature. But the lower quantum yield hinders its widespread use as an integrated quantum sensor. Here, we demonstrate an emission enhancement amounting to 400 by nanotrench arrays compatible with coplanar waveguide (CPW) electrodes employed for spin-state detection. By monitoring the reflectance spectrum of the resonators as additional layers of hBN are transferred, we have optimized the overall hBN/nanotrench optical response, maximizing thereby the luminescence enhancement. Based on these finely tuned heterostructures, we achieved an enhanced DC magnetic field sensitivity as high as 6 × 10-5 T/Hz1/2. Agency for Science, Technology and Research (A*STAR) National Research Foundation (NRF) Submitted/Accepted version This research is supported by the National Research Foundsation, Singapore, and A*STAR under its Quantum Engineering Programme (No. NRF2021-QEP2-03-P09, NRF2021-QEP2-01-P02, NRF2021-QEP2-01-P01, NRF2021-QEP2-03-P01, No. NRF2021-QEP2-03-P10, NRF2022-QEP2-02-P13) and IRG programme (M21K2c0116). 2023-10-13T00:52:53Z 2023-10-13T00:52:53Z 2023 Journal Article Cai, H., Ru, S., Jiang, Z., Eng, J. J. H., He, R., Li, F., Miao, Y., Zúñiga-Pérez, J. & Gao, W. (2023). Spin defects in hBN assisted by metallic nanotrenches for quantum sensing. Nano Letters, 23(11), 4991-4996. https://dx.doi.org/10.1021/acs.nanolett.3c00849 1530-6984 https://hdl.handle.net/10356/171095 10.1021/acs.nanolett.3c00849 37205843 2-s2.0-85162833679 11 23 4991 4996 en NRF2021-QEP2-03-P09 NRF2021-QEP2-01-P02 NRF2021-QEP2-01-P01 NRF2021-QEP2-03-P01 NRF2021-QEP2-03-P10 NRF2022-QEP2-02-P13 M21K2c0116 Nano Letters © 2023 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acs.nanolett.3c00849. application/pdf |
institution |
Nanyang Technological University |
building |
NTU Library |
continent |
Asia |
country |
Singapore Singapore |
content_provider |
NTU Library |
collection |
DR-NTU |
language |
English |
topic |
Science::Physics Hexagonal Boron Nitride Tunable Plasmonic |
spellingShingle |
Science::Physics Hexagonal Boron Nitride Tunable Plasmonic Cai, Hongbing Ru, Shihao Jiang, Zhengzhi Eng, John Jun Hong He, Ruihua Li, Fuli Miao, Yansong Zúñiga-Pérez, Jesús Gao, Weibo Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
description |
The omnipresence of hexagonal boron nitride (hBN) in devices embedding two-dimensional materials has prompted it as the most sought after platform to implement quantum sensing due to its testing while operating capability. The negatively charged boron vacancy (VB-) in hBN plays a prominent role, as it can be easily generated while its spin population can be initialized and read out by optical means at room-temperature. But the lower quantum yield hinders its widespread use as an integrated quantum sensor. Here, we demonstrate an emission enhancement amounting to 400 by nanotrench arrays compatible with coplanar waveguide (CPW) electrodes employed for spin-state detection. By monitoring the reflectance spectrum of the resonators as additional layers of hBN are transferred, we have optimized the overall hBN/nanotrench optical response, maximizing thereby the luminescence enhancement. Based on these finely tuned heterostructures, we achieved an enhanced DC magnetic field sensitivity as high as 6 × 10-5 T/Hz1/2. |
author2 |
School of Physical and Mathematical Sciences |
author_facet |
School of Physical and Mathematical Sciences Cai, Hongbing Ru, Shihao Jiang, Zhengzhi Eng, John Jun Hong He, Ruihua Li, Fuli Miao, Yansong Zúñiga-Pérez, Jesús Gao, Weibo |
format |
Article |
author |
Cai, Hongbing Ru, Shihao Jiang, Zhengzhi Eng, John Jun Hong He, Ruihua Li, Fuli Miao, Yansong Zúñiga-Pérez, Jesús Gao, Weibo |
author_sort |
Cai, Hongbing |
title |
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
title_short |
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
title_full |
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
title_fullStr |
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
title_full_unstemmed |
Spin defects in hBN assisted by metallic nanotrenches for quantum sensing |
title_sort |
spin defects in hbn assisted by metallic nanotrenches for quantum sensing |
publishDate |
2023 |
url |
https://hdl.handle.net/10356/171095 |
_version_ |
1781793903470444544 |