DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride

Spin defects existing in van der Waals materials attract wide attention thanks to their natural advantages for in situ quantum sensing, especially the negatively charged boron vacancy (VB-) centers in hexagonal boron nitride (h-BN). Here we systematically investigate the laser and microwave power br...

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Main Authors: Zhou, Feifei, Jiang, Zhengzhi, Liang, Haidong, Ru, Shihao, Bettiol, Andrew A., Gao, Weibo
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/171418
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1714182023-10-25T05:31:25Z DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride Zhou, Feifei Jiang, Zhengzhi Liang, Haidong Ru, Shihao Bettiol, Andrew A. Gao, Weibo School of Physical and Mathematical Sciences Science::Physics Hexagonal Boron Nitride Negatively Charged Boron Vacancy Centers Spin defects existing in van der Waals materials attract wide attention thanks to their natural advantages for in situ quantum sensing, especially the negatively charged boron vacancy (VB-) centers in hexagonal boron nitride (h-BN). Here we systematically investigate the laser and microwave power broadening in continuous-wave optically detected magnetic resonance (ODMR) of the VB- ensemble in h-BN, by revealing the behaviors of ODMR contrast and line width as a function of the laser and microwave powers. The experimental results are well explained by employing a two-level simplified model of ODMR dynamics. Furthermore, with optimized power, the DC magnetic field sensitivity of VB- ensemble is significantly improved up to 2.87 ± 0.07 μT/Hz. Our results provide important suggestions for further applications of VB- centers in quantum information processing and ODMR-based quantum sensing. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) National Research Foundation (NRF) This work is supported by Singapore Quantum engineering program (NRF2021-QEP2-01-P01, NRF2021-QEP2-01-P02, NRF2021-QEP2-03-P01, NRF2021-QEP2-03-P10, NRF2021-QEP2-03-P11), ASTAR IRG(M21K2c0116), and Singapore Ministry of Education (MOE2016-T3-1-006(S)) and Tier 2 Grant (MOE-T2EP50221-0009). 2023-10-25T05:31:25Z 2023-10-25T05:31:25Z 2023 Journal Article Zhou, F., Jiang, Z., Liang, H., Ru, S., Bettiol, A. A. & Gao, W. (2023). DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride. Nano Letters, 23(13), 6209-6215. https://dx.doi.org/10.1021/acs.nanolett.3c01881 1530-6984 https://hdl.handle.net/10356/171418 10.1021/acs.nanolett.3c01881 37364230 2-s2.0-85164287976 13 23 6209 6215 en NRF2021-QEP2-01-P01 NRF2021-QEP2-01-P02 NRF2021-QEP2-03-P01 NRF2021-QEP2-03-P10 NRF2021-QEP2-03-P11 M21K2c0116 MOE2016-T3-1-006(S) MOE-T2EP50221-0009 Nano Letters © 2023 American chemical Society. All rights reserved.
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Hexagonal Boron Nitride
Negatively Charged Boron Vacancy Centers
spellingShingle Science::Physics
Hexagonal Boron Nitride
Negatively Charged Boron Vacancy Centers
Zhou, Feifei
Jiang, Zhengzhi
Liang, Haidong
Ru, Shihao
Bettiol, Andrew A.
Gao, Weibo
DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
description Spin defects existing in van der Waals materials attract wide attention thanks to their natural advantages for in situ quantum sensing, especially the negatively charged boron vacancy (VB-) centers in hexagonal boron nitride (h-BN). Here we systematically investigate the laser and microwave power broadening in continuous-wave optically detected magnetic resonance (ODMR) of the VB- ensemble in h-BN, by revealing the behaviors of ODMR contrast and line width as a function of the laser and microwave powers. The experimental results are well explained by employing a two-level simplified model of ODMR dynamics. Furthermore, with optimized power, the DC magnetic field sensitivity of VB- ensemble is significantly improved up to 2.87 ± 0.07 μT/Hz. Our results provide important suggestions for further applications of VB- centers in quantum information processing and ODMR-based quantum sensing.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Zhou, Feifei
Jiang, Zhengzhi
Liang, Haidong
Ru, Shihao
Bettiol, Andrew A.
Gao, Weibo
format Article
author Zhou, Feifei
Jiang, Zhengzhi
Liang, Haidong
Ru, Shihao
Bettiol, Andrew A.
Gao, Weibo
author_sort Zhou, Feifei
title DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
title_short DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
title_full DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
title_fullStr DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
title_full_unstemmed DC magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
title_sort dc magnetic field sensitivity optimization of spin defects in hexagonal boron nitride
publishDate 2023
url https://hdl.handle.net/10356/171418
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