Orbital coupling of hetero-diatomic nickel-iron site for bifunctional electrocatalysis of CO₂ reduction and oxygen evolution

• Main Authors: Zeng, Zhiping, Gan, Liyong, Yang, Hongbin, Su, Xiaozhi, Gao, Jiajian, Liu, Wei, Matsumoto, Hiroaki, Gong, Jun, Zhang, Junming, Cai, Weizhen, Zhang, Zheye, Yan, Yibo, Liu, Bin, Chen, Peng
• Other Authors: School of Chemistry, Chemical Engineering and Biotechnology
• Format: Article
• Language: English
• Published: 2023
• Subjects: Engineering::Chemical engineering; Carbon Dioxide; Catalysis
• Online Access: https://hdl.handle.net/10356/172407
• Institution: Nanyang Technological University

While inheriting the exceptional merits of single atom catalysts, diatomic site catalysts (DASCs) utilize two adjacent atomic metal species for their complementary functionalities and synergistic actions. Herein, a DASC consisting of nickel-iron hetero-diatomic pairs anchored on nitrogen-doped graph...