Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles
Wearable smart textiles are natural carriers to enable imperceptible and highly permeable sensing and response to environmental conditions via the system integration of multiple functional fibers. However, the existing massive interfaces between different functional fibers significantly increase the...
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sg-ntu-dr.10356-1730792024-01-12T15:41:37Z Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles Liu, Fan Xu, Shuhong Gong, Wenbin Zhao, Kaitian Wang, Zhimin Luo, Jie Li, Chunsheng Sun, Yan Xue, Pan Wang, Chunlei Wei, Lei Li, Qingwen Zhang, Qichong School of Electrical and Electronic Engineering Engineering::Electrical and electronic engineering Aqueous Zinc-Ion Battery Carbon Dots Wearable smart textiles are natural carriers to enable imperceptible and highly permeable sensing and response to environmental conditions via the system integration of multiple functional fibers. However, the existing massive interfaces between different functional fibers significantly increase the complexity and reduce the wearability of the textile system. Thus, it is significant yet challenging to achieve all-in-one multifunctional fibers for realizing miniaturized and lightweight smart textiles with high reliability. Herein, as bifunctional electrolyte additives, fluorescent carbon dots with abundant zincophilic functional groups are introduced into electrolytes to develop fluorescent fiber-shaped aqueous zinc-ion batteries (FFAZIBs). Originating from effective dendrite suppression of Zn anodes and multiple active sites of freestanding Prussian blue cathodes, high energy density (0.17 Wh·cm-3) and long-term cyclability (78.9% capacity retention after 1500 cycles) are achieved for FFAZIBs. More importantly, the one-dimensional structure ensures the same luminance in all directions of FFAZIBs, enabling the form of multicolor display-in-battery textiles. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Nanyang Technological University National Research Foundation (NRF) Submitted/Accepted version This work was supported by the Natural Science Foundation of Jiangsu Province (BK20220288), the National Key R&D Program of China (2022YFA1203304), Natural Science Foundation of China (Grant Nos. 22075043 and 21875034), Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences (Start-up grant E1552102), the Singapore Ministry of Education Academic Research Fund Tier 2 (MOE2019-T2-2-127 and MOE-T2EP50120-0002), A*STAR under AME IRG (A2083c0062), and the Singapore National Research Foundation Competitive Research Program (NRF-CRP18-2017-02). This work was supported by A*STAR under its IAF-ICP Programme I2001E0067 and the Schaeffler Hub for Advanced Research at NTU. This work was also supported by NTU-PSL Joint Lab collaboration. This work was also supported by China Scholarship Council. 2024-01-10T08:05:32Z 2024-01-10T08:05:32Z 2023 Journal Article Liu, F., Xu, S., Gong, W., Zhao, K., Wang, Z., Luo, J., Li, C., Sun, Y., Xue, P., Wang, C., Wei, L., Li, Q. & Zhang, Q. (2023). Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles. ACS Nano, 17(18), 18494-18506. https://dx.doi.org/10.1021/acsnano.3c06245 1936-0851 https://hdl.handle.net/10356/173079 10.1021/acsnano.3c06245 37698337 2-s2.0-85172425989 18 17 18494 18506 en MOE2019-T2-2-127 MOE-T2EP50120-0002 A2083c0062 NRF-CRP18-2017-02 I2001E0067 ACS Nano © 2023 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acsnano.3c06245. application/pdf |
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Engineering::Electrical and electronic engineering Aqueous Zinc-Ion Battery Carbon Dots |
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Engineering::Electrical and electronic engineering Aqueous Zinc-Ion Battery Carbon Dots Liu, Fan Xu, Shuhong Gong, Wenbin Zhao, Kaitian Wang, Zhimin Luo, Jie Li, Chunsheng Sun, Yan Xue, Pan Wang, Chunlei Wei, Lei Li, Qingwen Zhang, Qichong Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
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Wearable smart textiles are natural carriers to enable imperceptible and highly permeable sensing and response to environmental conditions via the system integration of multiple functional fibers. However, the existing massive interfaces between different functional fibers significantly increase the complexity and reduce the wearability of the textile system. Thus, it is significant yet challenging to achieve all-in-one multifunctional fibers for realizing miniaturized and lightweight smart textiles with high reliability. Herein, as bifunctional electrolyte additives, fluorescent carbon dots with abundant zincophilic functional groups are introduced into electrolytes to develop fluorescent fiber-shaped aqueous zinc-ion batteries (FFAZIBs). Originating from effective dendrite suppression of Zn anodes and multiple active sites of freestanding Prussian blue cathodes, high energy density (0.17 Wh·cm-3) and long-term cyclability (78.9% capacity retention after 1500 cycles) are achieved for FFAZIBs. More importantly, the one-dimensional structure ensures the same luminance in all directions of FFAZIBs, enabling the form of multicolor display-in-battery textiles. |
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School of Electrical and Electronic Engineering |
author_facet |
School of Electrical and Electronic Engineering Liu, Fan Xu, Shuhong Gong, Wenbin Zhao, Kaitian Wang, Zhimin Luo, Jie Li, Chunsheng Sun, Yan Xue, Pan Wang, Chunlei Wei, Lei Li, Qingwen Zhang, Qichong |
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Article |
author |
Liu, Fan Xu, Shuhong Gong, Wenbin Zhao, Kaitian Wang, Zhimin Luo, Jie Li, Chunsheng Sun, Yan Xue, Pan Wang, Chunlei Wei, Lei Li, Qingwen Zhang, Qichong |
author_sort |
Liu, Fan |
title |
Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
title_short |
Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
title_full |
Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
title_fullStr |
Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
title_full_unstemmed |
Fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
title_sort |
fluorescent fiber-shaped aqueous zinc-ion batteries for bifunctional multicolor-emission/energy-storage textiles |
publishDate |
2024 |
url |
https://hdl.handle.net/10356/173079 |
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1789483051974131712 |