Surface-degenerate semiconductor photocatalysis for efficient water splitting without sacrificial agents via a reticular chemistry approach

• Main Authors: Ng, Li Shiuan, Raja Mogan, Tharishinny, Lee, Jinn-Kye, Li, Haitao, Lee, Ken Chi-Lik, Lee, Hiang Kwee
• Other Authors: School of Chemistry, Chemical Engineering and Biotechnology
• Format: Article
• Language: English
• Published: 2024
• Subjects: Engineering::Chemical engineering; Metal–Organic Framework; Nanoparticles
• Online Access: https://hdl.handle.net/10356/173095
• Institution: Nanyang Technological University

The production of green hydrogen through photocatalytic water splitting is crucial for a sustainable hydrogen economy and chemical manufacturing. However, current approaches suffer from slow hydrogen production (<70 μmol ⋅ gcat -1 ⋅ h-1 ) due to the sluggish four-electrons oxygen evolution react...