Contracted description of driven degenerate multilevel quantum systems

We formulate a contraction theorem that maps quantum dynamics of a multilevel degenerate system (DS) driven by a time-dependent external field to the dynamics of the corresponding contracted non-degenerate system (CNS) of lower dimension, provided transitions between each pair of degenerate levels i...

Full description

Saved in:
Bibliographic Details
Main Authors: Xu, Xiangyu, Sun, Kewei, Gelin, Maxim F., Zhao, Yang
Other Authors: School of Materials Science and Engineering
Format: Article
Language:English
Published: 2024
Subjects:
Online Access:https://hdl.handle.net/10356/173778
Tags: Add Tag
No Tags, Be the first to tag this record!
Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-173778
record_format dspace
spelling sg-ntu-dr.10356-1737782024-03-01T15:46:21Z Contracted description of driven degenerate multilevel quantum systems Xu, Xiangyu Sun, Kewei Gelin, Maxim F. Zhao, Yang School of Materials Science and Engineering Engineering Degenerate levels External fields We formulate a contraction theorem that maps quantum dynamics of a multilevel degenerate system (DS) driven by a time-dependent external field to the dynamics of the corresponding contracted non-degenerate system (CNS) of lower dimension, provided transitions between each pair of degenerate levels in the DS have identical transition dipole moments. The theorem is valid for an external field of any strength and shape, with and without rotating wave approximation in the system-field interaction. It establishes explicit relations between DS and CNS observables, significantly simplifies numerical calculations, and clarifies physical origins of the field-induced DS dynamics. Ministry of Education (MOE) Published version Support from the Singapore Ministry of Education Academic Research Fund Tier 1 (Grant No. RG87/20) is gratefully acknowledged. K.S. and M.F.G. acknowledge support from Hangzhou Dianzi University through startup funding. 2024-02-27T02:08:49Z 2024-02-27T02:08:49Z 2023 Journal Article Xu, X., Sun, K., Gelin, M. F. & Zhao, Y. (2023). Contracted description of driven degenerate multilevel quantum systems. Journal of Chemical Physics, 159(22). https://dx.doi.org/10.1063/5.0178460 0021-9606 https://hdl.handle.net/10356/173778 10.1063/5.0178460 38088431 2-s2.0-85179648937 22 159 en RG87/20 Journal of Chemical Physics © 2023 Author(s). Published under an exclusive license by AIP Publishing. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1063/5.0178460 application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering
Degenerate levels
External fields
spellingShingle Engineering
Degenerate levels
External fields
Xu, Xiangyu
Sun, Kewei
Gelin, Maxim F.
Zhao, Yang
Contracted description of driven degenerate multilevel quantum systems
description We formulate a contraction theorem that maps quantum dynamics of a multilevel degenerate system (DS) driven by a time-dependent external field to the dynamics of the corresponding contracted non-degenerate system (CNS) of lower dimension, provided transitions between each pair of degenerate levels in the DS have identical transition dipole moments. The theorem is valid for an external field of any strength and shape, with and without rotating wave approximation in the system-field interaction. It establishes explicit relations between DS and CNS observables, significantly simplifies numerical calculations, and clarifies physical origins of the field-induced DS dynamics.
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Xu, Xiangyu
Sun, Kewei
Gelin, Maxim F.
Zhao, Yang
format Article
author Xu, Xiangyu
Sun, Kewei
Gelin, Maxim F.
Zhao, Yang
author_sort Xu, Xiangyu
title Contracted description of driven degenerate multilevel quantum systems
title_short Contracted description of driven degenerate multilevel quantum systems
title_full Contracted description of driven degenerate multilevel quantum systems
title_fullStr Contracted description of driven degenerate multilevel quantum systems
title_full_unstemmed Contracted description of driven degenerate multilevel quantum systems
title_sort contracted description of driven degenerate multilevel quantum systems
publishDate 2024
url https://hdl.handle.net/10356/173778
_version_ 1794549402035027968