Finite-temperature hole–magnon dynamics in an antiferromagnet
Employing the numerically accurate multiple Davydov Ansatz in combination with the thermo-field dynamics approach, we delve into the interplay of the finite-temperature dynamics of holes and magnons in an antiferromagnet, which allows for scrutinizing previous predictions from the self-consistent Bo...
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sg-ntu-dr.10356-1746642024-04-12T15:48:06Z Finite-temperature hole–magnon dynamics in an antiferromagnet Shen, Kaijun Sun, Kewei Gelin, Maxim F. Zhao, Yang School of Materials Science and Engineering Engineering Antiferromagnetic materials Temperature distribution Employing the numerically accurate multiple Davydov Ansatz in combination with the thermo-field dynamics approach, we delve into the interplay of the finite-temperature dynamics of holes and magnons in an antiferromagnet, which allows for scrutinizing previous predictions from the self-consistent Born approximation while offering, for the first time, accurate finite-temperature computation of detailed magnon dynamics as a response and a facilitator to the hole motion. The study also uncovers a pronounced temperature dependence of the magnon and hole populations, pointing to the feasibility of potential thermal manipulation and control of hole dynamics. Our methodology can be applied not only to the calculation of steady-state angular-resolved photoemission spectra but also to the simulation of femtosecond terahertz pump-probe and other nonlinear signals for the characterization of antiferromagnetic materials. Ministry of Education (MOE) Submitted/Accepted version The authors gratefully acknowledge the support of the Singapore Ministry of Education Academic Research Fund (Grant No. RG87/20). K. Sun would also like to thank the Natural Science Foundation of Zhejiang Province (Grant No. LY18A040005) for partial support. M.F.G. acknowledges the support of Hangzhou Dianzi University through startup funding. 2024-04-07T05:19:05Z 2024-04-07T05:19:05Z 2024 Journal Article Shen, K., Sun, K., Gelin, M. F. & Zhao, Y. (2024). Finite-temperature hole–magnon dynamics in an antiferromagnet. Journal of Physical Chemistry Letters, 15(2), 447-453. https://dx.doi.org/10.1021/acs.jpclett.3c03298 1948-7185 https://hdl.handle.net/10356/174664 10.1021/acs.jpclett.3c03298 38189682 2-s2.0-85182563372 http://arxiv.org/abs/2401.11184v1 2 15 447 453 en RG87/20 Journal of Physical Chemistry Letters © 2024 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acs.jpclett.3c03298. application/pdf |
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Engineering Antiferromagnetic materials Temperature distribution Shen, Kaijun Sun, Kewei Gelin, Maxim F. Zhao, Yang Finite-temperature hole–magnon dynamics in an antiferromagnet |
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Employing the numerically accurate multiple Davydov Ansatz in combination with the thermo-field dynamics approach, we delve into the interplay of the finite-temperature dynamics of holes and magnons in an antiferromagnet, which allows for scrutinizing previous predictions from the self-consistent Born approximation while offering, for the first time, accurate finite-temperature computation of detailed magnon dynamics as a response and a facilitator to the hole motion. The study also uncovers a pronounced temperature dependence of the magnon and hole populations, pointing to the feasibility of potential thermal manipulation and control of hole dynamics. Our methodology can be applied not only to the calculation of steady-state angular-resolved photoemission spectra but also to the simulation of femtosecond terahertz pump-probe and other nonlinear signals for the characterization of antiferromagnetic materials. |
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School of Materials Science and Engineering |
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School of Materials Science and Engineering Shen, Kaijun Sun, Kewei Gelin, Maxim F. Zhao, Yang |
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Article |
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Shen, Kaijun Sun, Kewei Gelin, Maxim F. Zhao, Yang |
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Shen, Kaijun |
title |
Finite-temperature hole–magnon dynamics in an antiferromagnet |
title_short |
Finite-temperature hole–magnon dynamics in an antiferromagnet |
title_full |
Finite-temperature hole–magnon dynamics in an antiferromagnet |
title_fullStr |
Finite-temperature hole–magnon dynamics in an antiferromagnet |
title_full_unstemmed |
Finite-temperature hole–magnon dynamics in an antiferromagnet |
title_sort |
finite-temperature hole–magnon dynamics in an antiferromagnet |
publishDate |
2024 |
url |
https://hdl.handle.net/10356/174664 http://arxiv.org/abs/2401.11184v1 |
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1800916413071753216 |