The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations

The speed at which crystals settle in magmatic reservoirs affects the solidification rate of magmas and their differentiation. Despite extensive prior work on the subject, most of our quantitative understanding of the process is still restricted to treating crystals as spherical particles and does n...

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Main Authors: Mourey, Adrien J., Carrara, Alexandre, Shea, Thomas, Costa, Fidel, Longpré, Marc-Antoine
Other Authors: Asian School of the Environment
Format: Article
Language:English
Published: 2024
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Online Access:https://hdl.handle.net/10356/174729
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Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-174729
record_format dspace
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Earth and Environmental Sciences
Olivine
Crystal settling
spellingShingle Earth and Environmental Sciences
Olivine
Crystal settling
Mourey, Adrien J.
Carrara, Alexandre
Shea, Thomas
Costa, Fidel
Longpré, Marc-Antoine
The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
description The speed at which crystals settle in magmatic reservoirs affects the solidification rate of magmas and their differentiation. Despite extensive prior work on the subject, most of our quantitative understanding of the process is still restricted to treating crystals as spherical particles and does not address the geometric complexities of natural crystals. Here, we use three-dimensional (3D) X-ray microcomputed tomography (X-μCT) observations on olivine crystals from Kīlauea Volcano (Hawai‘i) to document their highly intricate and variable geometries, and the textural growth relationships between the olivine crystals and their inclusions (melt, spinel, and fluid/vapor bubbles). Olivine crystals generally have clustered polyhedral or skeletal shapes, which reflect variable magmatic conditions (or growth rates) during their formation. The cumulative presence of spinel, melt, fluid, and vapor inclusions affects the density of the host crystals by up to 6% relative, and thus plays a limited role on modifying crystal settling rate. In contrast, the overall crystal shape plays a major role. We performed numerical simulations employing a finite element method to investigate the effect of crystal morphology on settling rate and the evolution of the particle volume fraction in a magmatic convective layer. We show that for all olivine geometries investigated, the settling velocity is highest when the long axis of the crystal is aligned with the flow direction of the melt. Increasing the aspect ratio of the olivine tends to decrease its settling velocity and results in an increase in the influence of its orientation on the terminal velocity (UT). Extrapolation of the simulation results to variable particle volume fractions (Φ = 0–0.5) indicates high crystal settling rates (UT = ∼9.7 × 10−6–1.4 × 10−5 m/s) that are used to estimate the timescales for the formation of olivine cumulates in natural melt-dominated basaltic systems. The formation of olivine cumulates is therefore rapid, potentially leading to the accumulation of a crystal layer at the bottom, where the frictional contacts between the crystals exert a rheological lock-up acting against further convection. Crystal accumulation in the locked layer (parametrized with the solid/liquid volume ratio in the reservoir) is a function of the reservoir size and crystal fraction, and takes a few years in small reservoirs (<1 km thick) and a few decades in larger reservoirs (several kms thick). We propose a calibration of olivine suspension timescales for mafic magma reservoirs (based on the knowledge of the particle volume fraction, reservoir height, and olivine morphology). This calibration is used to estimate the rate of cumulate build-up, and can help interpret crystal size distributions in the framework of crystal suspension times.
author2 Asian School of the Environment
author_facet Asian School of the Environment
Mourey, Adrien J.
Carrara, Alexandre
Shea, Thomas
Costa, Fidel
Longpré, Marc-Antoine
format Article
author Mourey, Adrien J.
Carrara, Alexandre
Shea, Thomas
Costa, Fidel
Longpré, Marc-Antoine
author_sort Mourey, Adrien J.
title The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
title_short The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
title_full The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
title_fullStr The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
title_full_unstemmed The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
title_sort influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations
publishDate 2024
url https://hdl.handle.net/10356/174729
_version_ 1814047051026006016
spelling sg-ntu-dr.10356-1747292024-04-08T15:30:48Z The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations Mourey, Adrien J. Carrara, Alexandre Shea, Thomas Costa, Fidel Longpré, Marc-Antoine Asian School of the Environment Earth Observatory of Singapore Earth and Environmental Sciences Olivine Crystal settling The speed at which crystals settle in magmatic reservoirs affects the solidification rate of magmas and their differentiation. Despite extensive prior work on the subject, most of our quantitative understanding of the process is still restricted to treating crystals as spherical particles and does not address the geometric complexities of natural crystals. Here, we use three-dimensional (3D) X-ray microcomputed tomography (X-μCT) observations on olivine crystals from Kīlauea Volcano (Hawai‘i) to document their highly intricate and variable geometries, and the textural growth relationships between the olivine crystals and their inclusions (melt, spinel, and fluid/vapor bubbles). Olivine crystals generally have clustered polyhedral or skeletal shapes, which reflect variable magmatic conditions (or growth rates) during their formation. The cumulative presence of spinel, melt, fluid, and vapor inclusions affects the density of the host crystals by up to 6% relative, and thus plays a limited role on modifying crystal settling rate. In contrast, the overall crystal shape plays a major role. We performed numerical simulations employing a finite element method to investigate the effect of crystal morphology on settling rate and the evolution of the particle volume fraction in a magmatic convective layer. We show that for all olivine geometries investigated, the settling velocity is highest when the long axis of the crystal is aligned with the flow direction of the melt. Increasing the aspect ratio of the olivine tends to decrease its settling velocity and results in an increase in the influence of its orientation on the terminal velocity (UT). Extrapolation of the simulation results to variable particle volume fractions (Φ = 0–0.5) indicates high crystal settling rates (UT = ∼9.7 × 10−6–1.4 × 10−5 m/s) that are used to estimate the timescales for the formation of olivine cumulates in natural melt-dominated basaltic systems. The formation of olivine cumulates is therefore rapid, potentially leading to the accumulation of a crystal layer at the bottom, where the frictional contacts between the crystals exert a rheological lock-up acting against further convection. Crystal accumulation in the locked layer (parametrized with the solid/liquid volume ratio in the reservoir) is a function of the reservoir size and crystal fraction, and takes a few years in small reservoirs (<1 km thick) and a few decades in larger reservoirs (several kms thick). We propose a calibration of olivine suspension timescales for mafic magma reservoirs (based on the knowledge of the particle volume fraction, reservoir height, and olivine morphology). This calibration is used to estimate the rate of cumulate build-up, and can help interpret crystal size distributions in the framework of crystal suspension times. Submitted/Accepted version A.M. and T.S. received funding from the National Science Foundation (NSF) grant to T. S. (EAR 1725321). A.C. was partly supported by the National Science Foundation grant EAR-1950113, and the Region Auvergne and the European Regional Development Fund (Laboratory of Excellence ClerVolc contribution number 645). M.-A.L. was supported through NSF award EAR 1650379. 2024-04-08T07:20:38Z 2024-04-08T07:20:38Z 2024 Journal Article Mourey, A. J., Carrara, A., Shea, T., Costa, F. & Longpré, M. (2024). The influence of olivine settling on the formation of basaltic cumulates revealed by micro-tomography and numerical simulations. Journal of Volcanology and Geothermal Research, 449, 108051-. https://dx.doi.org/10.1016/j.jvolgeores.2024.108051 0377-0273 https://hdl.handle.net/10356/174729 10.1016/j.jvolgeores.2024.108051 2-s2.0-85188526272 449 108051 en Journal of Volcanology and Geothermal Research © 2024 Elsevier B.V. All rights reserved. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1016/j.jvolgeores.2024.108051. application/pdf