Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites

Co-encapsulation of endospores and nutrients in self-healing concrete can mitigate their negative effects on cement hydration. However, the current approaches of co-encapsulation for bacteria-based self-healing cementitious composites could cause pre-consumption of nutrients before cracking or a res...

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Main Authors: Feng, Jianhang, Dai, Xiaodi, Qian, Shunzhi
Other Authors: School of Civil and Environmental Engineering
Format: Article
Language:English
Published: 2024
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Online Access:https://hdl.handle.net/10356/180798
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1807982024-10-28T02:06:06Z Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites Feng, Jianhang Dai, Xiaodi Qian, Shunzhi School of Civil and Environmental Engineering Engineering Bacterial spores Co-encapsulation Co-encapsulation of endospores and nutrients in self-healing concrete can mitigate their negative effects on cement hydration. However, the current approaches of co-encapsulation for bacteria-based self-healing cementitious composites could cause pre-consumption of nutrients before cracking or a restricted release of nutrients after cracking. To address the nutrient release issue, polyethylene glycol (PEG) with high solubility was applied as an alternative to co-encapsulation of bacterial spores and nutrients, subsequently coated by an epoxy/sand protective shell herein. The core-shell structured capsules rapidly released the encapsulated substances within approximately 4 h and protected the encapsulated endospores in alkali environments. Due to the co-encapsulation, hydration retardation was avoided, leading to less severe reductions in compressive strength. After cracking, although the released amount of nutrients decreased after encapsulation, the closure of cracks below 300 μm was improved in the presence of capsules, thus water tightness was recovered more significantly. A model was developed to simulate sealing evolutions, and the modelling results were generally consistent with the experimental results. Ministry of Education (MOE) Nanyang Technological University The first author would like to appreciate the support of NTU PhD scholarship. The authors would like to acknowledge the financial support from the Ministry of Education, Singapore, under its Academic Research Fund Tier 1 (RG71/20). 2024-10-28T02:06:06Z 2024-10-28T02:06:06Z 2024 Journal Article Feng, J., Dai, X. & Qian, S. (2024). Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites. Cement and Concrete Composites, 153, 105713-. https://dx.doi.org/10.1016/j.cemconcomp.2024.105713 0958-9465 https://hdl.handle.net/10356/180798 10.1016/j.cemconcomp.2024.105713 2-s2.0-85201224033 153 105713 en RG71/20 Cement and Concrete Composites © 2024 Elsevier Ltd. All rights are reserved, including those for text and data mining, AI training, and similar technologies.
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering
Bacterial spores
Co-encapsulation
spellingShingle Engineering
Bacterial spores
Co-encapsulation
Feng, Jianhang
Dai, Xiaodi
Qian, Shunzhi
Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
description Co-encapsulation of endospores and nutrients in self-healing concrete can mitigate their negative effects on cement hydration. However, the current approaches of co-encapsulation for bacteria-based self-healing cementitious composites could cause pre-consumption of nutrients before cracking or a restricted release of nutrients after cracking. To address the nutrient release issue, polyethylene glycol (PEG) with high solubility was applied as an alternative to co-encapsulation of bacterial spores and nutrients, subsequently coated by an epoxy/sand protective shell herein. The core-shell structured capsules rapidly released the encapsulated substances within approximately 4 h and protected the encapsulated endospores in alkali environments. Due to the co-encapsulation, hydration retardation was avoided, leading to less severe reductions in compressive strength. After cracking, although the released amount of nutrients decreased after encapsulation, the closure of cracks below 300 μm was improved in the presence of capsules, thus water tightness was recovered more significantly. A model was developed to simulate sealing evolutions, and the modelling results were generally consistent with the experimental results.
author2 School of Civil and Environmental Engineering
author_facet School of Civil and Environmental Engineering
Feng, Jianhang
Dai, Xiaodi
Qian, Shunzhi
format Article
author Feng, Jianhang
Dai, Xiaodi
Qian, Shunzhi
author_sort Feng, Jianhang
title Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
title_short Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
title_full Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
title_fullStr Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
title_full_unstemmed Co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
title_sort co-encapsulation of bacterial spores and nutrients by polyethylene glycol for self-sealing cementitious composites
publishDate 2024
url https://hdl.handle.net/10356/180798
_version_ 1814777796434591744