Dynamic adaptation of active site driven by dual-side adsorptionin single-atomic catalysts during CO2 electroreduction

• Main Authors: Tran, Nam Van, Liu, Jiyuan, Li, Shuzhou
• Other Authors: School of Materials Science and Engineering
• Format: Article
• Language: English
• Published: 2025
• Subjects: Engineering; CO2 electroreduction; Single-atomic catalysts
• Online Access: https://hdl.handle.net/10356/181971
• Institution: Nanyang Technological University

Single-atom iron embedded in N-doped carbon (Fe-N-C) is among the most representative single-atomic catalysts (SACs) for electrochemical CO2 reduction reaction (CO2RR). Despite the simplicity of the active site, the CO2-to-CO mechanism on Fe-N-C remains controversial. Firstly, there is a long debate...