High-entropy effect breaking the oxo wall for selective high-valent metal–oxo species generation

• Main Authors: Shi, Zhonglian, Li, Chao, Liu, Wei, Jiang, Ziyi, Chen, Haohao, Kong, Xin Ying, Wang, Li, Huang, Yingping, Xia, Dehua, Ye, Liqun
• Other Authors: School of Chemistry, Chemical Engineering and Biotechnology
• Format: Article
• Language: English
• Published: 2025
• Subjects: Chemistry; High-entropy; Electron delocalization
• Online Access: https://hdl.handle.net/10356/182087
• Institution: Nanyang Technological University

The advancement of multiphase catalysts that consist of multiple active sites is the key to improving the catalytic activity of peroxymonosulfate (PMS)-based Fenton catalysts. However, enormous challenges remain in rationally regulating the electronic configuration of each metal center to further im...