Van Hove annihilation and nematic instability on a kagome lattice

A nematic phase breaks the point-group symmetry of the crystal lattice and is known to emerge in correlated materials. Here we report the observation of an intra-unit-cell nematic order and associated Fermi surface deformation in the kagome metal ScV6Sn6. Using scanning tunnelling microscopy and sca...

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Main Authors: Jiang, Yu-Xiao, Shao, Sen, Xia, Wei, Denner, M. Michael, Ingham, Julian, Hossain, Md Shafayat, Qiu, Qingzheng, Zheng, Xiquan, Chen, Hongyu, Cheng, Zi-Jia, Yang, Xian P., Kim, Byunghoon, Yin, Jia-Xin, Zhang, Songbo, Litskevich, Maksim, Zhang, Qi, Cochran, Tyler A., Peng, Yingying, Chang, Guoqing, Guo, Yanfeng, Thomale, Ronny, Neupert, Titus, Hasan, M. Zahid
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2025
Subjects:
Online Access:https://hdl.handle.net/10356/182713
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Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-182713
record_format dspace
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Physics
Kagome lattice
Nematics
spellingShingle Physics
Kagome lattice
Nematics
Jiang, Yu-Xiao
Shao, Sen
Xia, Wei
Denner, M. Michael
Ingham, Julian
Hossain, Md Shafayat
Qiu, Qingzheng
Zheng, Xiquan
Chen, Hongyu
Cheng, Zi-Jia
Yang, Xian P.
Kim, Byunghoon
Yin, Jia-Xin
Zhang, Songbo
Litskevich, Maksim
Zhang, Qi
Cochran, Tyler A.
Peng, Yingying
Chang, Guoqing
Guo, Yanfeng
Thomale, Ronny
Neupert, Titus
Hasan, M. Zahid
Van Hove annihilation and nematic instability on a kagome lattice
description A nematic phase breaks the point-group symmetry of the crystal lattice and is known to emerge in correlated materials. Here we report the observation of an intra-unit-cell nematic order and associated Fermi surface deformation in the kagome metal ScV6Sn6. Using scanning tunnelling microscopy and scanning tunnelling spectroscopy, we reveal a stripe-like nematic order breaking the crystal rotational symmetry within the kagome lattice itself. Moreover, we identify a set of Van Hove singularities adhering to the kagome-layer electrons, which appear along one direction of the Brillouin zone and are annihilated along other high-symmetry directions, revealing rotational symmetry breaking. Via detailed spectroscopic maps, we further observe an elliptical deformation of the Fermi surface, which provides direct evidence for an electronically mediated nematic order. Our work not only bridges the gap between electronic nematicity and kagome physics but also sheds light on the potential mechanism for realizing symmetry-broken phases in correlated electron systems.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Jiang, Yu-Xiao
Shao, Sen
Xia, Wei
Denner, M. Michael
Ingham, Julian
Hossain, Md Shafayat
Qiu, Qingzheng
Zheng, Xiquan
Chen, Hongyu
Cheng, Zi-Jia
Yang, Xian P.
Kim, Byunghoon
Yin, Jia-Xin
Zhang, Songbo
Litskevich, Maksim
Zhang, Qi
Cochran, Tyler A.
Peng, Yingying
Chang, Guoqing
Guo, Yanfeng
Thomale, Ronny
Neupert, Titus
Hasan, M. Zahid
format Article
author Jiang, Yu-Xiao
Shao, Sen
Xia, Wei
Denner, M. Michael
Ingham, Julian
Hossain, Md Shafayat
Qiu, Qingzheng
Zheng, Xiquan
Chen, Hongyu
Cheng, Zi-Jia
Yang, Xian P.
Kim, Byunghoon
Yin, Jia-Xin
Zhang, Songbo
Litskevich, Maksim
Zhang, Qi
Cochran, Tyler A.
Peng, Yingying
Chang, Guoqing
Guo, Yanfeng
Thomale, Ronny
Neupert, Titus
Hasan, M. Zahid
author_sort Jiang, Yu-Xiao
title Van Hove annihilation and nematic instability on a kagome lattice
title_short Van Hove annihilation and nematic instability on a kagome lattice
title_full Van Hove annihilation and nematic instability on a kagome lattice
title_fullStr Van Hove annihilation and nematic instability on a kagome lattice
title_full_unstemmed Van Hove annihilation and nematic instability on a kagome lattice
title_sort van hove annihilation and nematic instability on a kagome lattice
publishDate 2025
url https://hdl.handle.net/10356/182713
_version_ 1825619634728992768
spelling sg-ntu-dr.10356-1827132025-02-24T15:36:23Z Van Hove annihilation and nematic instability on a kagome lattice Jiang, Yu-Xiao Shao, Sen Xia, Wei Denner, M. Michael Ingham, Julian Hossain, Md Shafayat Qiu, Qingzheng Zheng, Xiquan Chen, Hongyu Cheng, Zi-Jia Yang, Xian P. Kim, Byunghoon Yin, Jia-Xin Zhang, Songbo Litskevich, Maksim Zhang, Qi Cochran, Tyler A. Peng, Yingying Chang, Guoqing Guo, Yanfeng Thomale, Ronny Neupert, Titus Hasan, M. Zahid School of Physical and Mathematical Sciences Physics Kagome lattice Nematics A nematic phase breaks the point-group symmetry of the crystal lattice and is known to emerge in correlated materials. Here we report the observation of an intra-unit-cell nematic order and associated Fermi surface deformation in the kagome metal ScV6Sn6. Using scanning tunnelling microscopy and scanning tunnelling spectroscopy, we reveal a stripe-like nematic order breaking the crystal rotational symmetry within the kagome lattice itself. Moreover, we identify a set of Van Hove singularities adhering to the kagome-layer electrons, which appear along one direction of the Brillouin zone and are annihilated along other high-symmetry directions, revealing rotational symmetry breaking. Via detailed spectroscopic maps, we further observe an elliptical deformation of the Fermi surface, which provides direct evidence for an electronically mediated nematic order. Our work not only bridges the gap between electronic nematicity and kagome physics but also sheds light on the potential mechanism for realizing symmetry-broken phases in correlated electron systems. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Nanyang Technological University National Research Foundation (NRF) Submitted/Accepted version The M.Z.H. group acknowledges primary support from the US Department of Energy, Ofice of Science, National Quantum Information Science Research Centers, Quantum Science Center (at Oak Ridge National Laboratory) and Princeton University; scanning tunneling microscopy instrumentation support from the Gordon and Betty Moore Foundation (GBMF9461) and support with theory work; and support from the US Department of Energy under the Basic Energy Sciences program (grant no. DOE/BES DE-FG-02-05ER46200) for the theory and sample characterization work, including photoemission spectroscopy. Work at Nanyang Technological University was supported by the National Research Foundation, Singapore, under its Fellowship Award (NRF-NRFF13-2021-0010), the Agency for Science, Technology and Research (A*STAR) under its Manufacturing, Trade and Connectivity Individual Research Grant (grant no. M23M6c0100), the Singapore Ministry of Education AcRF Tier 2 grant (MOE-T2EP50222-0014) and the Nanyang Assistant Professorship grant (NTU-SUG). The computational work at Nanyang Technological University for this article was partially performed on resources of the National Supercomputing Centre, Singapore (https://www.nscc.sg). T.N., M.M.D. and S.Z. were supported by the European Research Council under the European Union’s Horizon 2020 research and innovation programme (ERC-StG-Neupert757867-PARATOP). S.Z. was also supported by the UZH Postdoc Grant. R.T. was supported by the Deutsche Forschungsgemeinschaft (German Research Foundation) through Project-ID 258499086-SFB 1170 and the Wurzburg-Dresden Cluster of Excellence on Complexity and Topology in Quantum Matter–ct.qmat Project-ID 390858490-EXC 2147. Y.G. acknowledges the Double First-Class Initiative Fund of ShanghaiTech University. W.X. acknowledges the research fund from the State Key Laboratory of Surface Physics and Department of Physics, Fudan University (grant no. KF2022_13). Y.P. is grateful for financial support from the National Natural Science Foundation of China (grant no. 12374143). 2025-02-18T07:27:55Z 2025-02-18T07:27:55Z 2024 Journal Article Jiang, Y., Shao, S., Xia, W., Denner, M. M., Ingham, J., Hossain, M. S., Qiu, Q., Zheng, X., Chen, H., Cheng, Z., Yang, X. P., Kim, B., Yin, J., Zhang, S., Litskevich, M., Zhang, Q., Cochran, T. A., Peng, Y., Chang, G., ...Hasan, M. Z. (2024). Van Hove annihilation and nematic instability on a kagome lattice. Nature Materials, 23(9), 1214-1221. https://dx.doi.org/10.1038/s41563-024-01914-z 1476-1122 https://hdl.handle.net/10356/182713 10.1038/s41563-024-01914-z 39009656 2-s2.0-85198640403 9 23 1214 1221 en NRF-NRFF13 2021-0010 M23M6c0100 MOE-T2EP50222-0014 NTU-SUG Nature Materials © 2024 The Author(s), under exclusive licence to Springer Nature Limited. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1038/s41563-024-01914-z application/pdf