A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks
Blue-color stimulated emission with low threshold power is observed from In- and Zn-MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal-ion centers in the solid state. The density-of-states and transition dipole moments are calculated and the stimulate...
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sg-ntu-dr.10356-802372023-02-28T19:31:37Z A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks Medishetty, Raghavender Nalla, Venkatram Nemec, Lydia Henke, Sebastian Mayer, David Sun, Handong Reuter, Karsten Fischer, Roland A. School of Physical and Mathematical Sciences Centre for Disruptive Photonic Technologies (CDPT) Stimulated emission Nonlinear optics Blue-color stimulated emission with low threshold power is observed from In- and Zn-MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal-ion centers in the solid state. The density-of-states and transition dipole moments are calculated and the stimulated emission phenomenon is correlated with these properties. MOE (Min. of Education, S’pore) Accepted version 2017-02-21T07:53:37Z 2019-12-06T13:45:33Z 2017-02-21T07:53:37Z 2019-12-06T13:45:33Z 2017 2017 Journal Article Medishetty, R., Nalla, V., Nemec, L., Henke, S., Mayer, D., Sun, H., et al. (2017). A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks. Advanced Materials, in press. 0935-9648 https://hdl.handle.net/10356/80237 http://hdl.handle.net/10220/42115 10.1002/adma.201605637 196048 en Advanced Materials © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is the author created version of a work that has been peer reviewed and accepted for publication by Advanced Materials, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [http://dx.doi.org/10.1002/adma.201605637]. 13 p. application/pdf image/png |
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Stimulated emission Nonlinear optics Medishetty, Raghavender Nalla, Venkatram Nemec, Lydia Henke, Sebastian Mayer, David Sun, Handong Reuter, Karsten Fischer, Roland A. A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
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Blue-color stimulated emission with low threshold power is observed from In- and Zn-MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal-ion centers in the solid state. The density-of-states and transition dipole moments are calculated and the stimulated emission phenomenon is correlated with these properties. |
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School of Physical and Mathematical Sciences |
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School of Physical and Mathematical Sciences Medishetty, Raghavender Nalla, Venkatram Nemec, Lydia Henke, Sebastian Mayer, David Sun, Handong Reuter, Karsten Fischer, Roland A. |
format |
Article |
author |
Medishetty, Raghavender Nalla, Venkatram Nemec, Lydia Henke, Sebastian Mayer, David Sun, Handong Reuter, Karsten Fischer, Roland A. |
author_sort |
Medishetty, Raghavender |
title |
A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
title_short |
A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
title_full |
A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
title_fullStr |
A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
title_full_unstemmed |
A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal-Organic Frameworks |
title_sort |
new class of lasing materials: intrinsic stimulated emission from nonlinear optically active metal-organic frameworks |
publishDate |
2017 |
url |
https://hdl.handle.net/10356/80237 http://hdl.handle.net/10220/42115 |
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1759854379477762048 |