Vibrational relaxation dynamics of the nitrogen-vacancy center in diamond

• Main Authors: Ulbricht, Ronald, Dong, Shuo, Gali, Adam, Meng, Sheng, Loh, Zhi-Heng
• 其他作者: School of Physical and Mathematical Sciences
• 格式: Article
• 語言: English
• 出版: 2018
• 主題: Vibrational Energy Relaxation; Nitrogen Vacancy; DRNTU::Science::Physics
• 在線閱讀: https://hdl.handle.net/10356/80429; http://hdl.handle.net/10220/46490
• 機構: Nanyang Technological University

We employ a combination of spectrally resolved optical pump-probe spectroscopy and excited-state ab initio molecular dynamics (ESAIMD) simulations to study the ultrafast vibrational relaxation dynamics of the 3E excited state of negatively charged nitrogen vacancy (NV−) defects. The experimental res...