Single-shot condensation of exciton polaritons and the hole burning effect

A bosonic condensate of exciton polaritons in a semiconductor microcavity is a macroscopic quantum state subject to pumping and decay. The fundamental nature of this driven-dissipative condensate is still under debate. Here, we gain an insight into spontaneous condensation by imaging long-lifetime e...

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Main Authors: Snoke, D. W., Truscott, A. G., Estrecho, E., Gao, T., Bobrovska, N., Fraser, M. D., Steger, M., Pfeiffer, L., West, K., Liew, Timothy Chi Hin, Matuszewski, M., Ostrovskaya, E. A.
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2018
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Online Access:https://hdl.handle.net/10356/89121
http://hdl.handle.net/10220/46076
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-891212023-02-28T19:23:57Z Single-shot condensation of exciton polaritons and the hole burning effect Snoke, D. W. Truscott, A. G. Estrecho, E. Gao, T. Bobrovska, N. Fraser, M. D. Steger, M. Pfeiffer, L. West, K. Liew, Timothy Chi Hin Matuszewski, M. Ostrovskaya, E. A. School of Physical and Mathematical Sciences DRNTU::Science::Physics Exciton Polaritons Single-shot Condensation A bosonic condensate of exciton polaritons in a semiconductor microcavity is a macroscopic quantum state subject to pumping and decay. The fundamental nature of this driven-dissipative condensate is still under debate. Here, we gain an insight into spontaneous condensation by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in a single-shot optical excitation regime, without averaging over multiple condensate realisations. We demonstrate that condensation is strongly influenced by an incoherent reservoir and that the reservoir depletion, the so-called spatial hole burning, is critical for the transition to the ground state. Condensates of photon-like polaritons exhibit strong shot-to-shot fluctuations and density filamentation due to the effective self-focusing associated with the reservoir depletion. In contrast, condensates of exciton-like polaritons display smoother spatial density distributions and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study fundamental properties of non-equilibrium condensation in the presence of a reservoir. MOE (Min. of Education, S’pore) Published version 2018-09-24T07:51:24Z 2019-12-06T17:18:20Z 2018-09-24T07:51:24Z 2019-12-06T17:18:20Z 2018 Journal Article Estrecho, E., Gao, T., Bobrovska, N., Fraser, M. D., Steger, M., Pfeiffer, L., . . . Ostrovskaya, E. A. (2018). Single-shot condensation of exciton polaritons and the hole burning effect. Nature Communications, 9(1), 2944-. doi:10.1038/s41467-018-05349-4 https://hdl.handle.net/10356/89121 http://hdl.handle.net/10220/46076 10.1038/s41467-018-05349-4 en Nature Communications © 2018 The Author(s). This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. 9 p. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic DRNTU::Science::Physics
Exciton Polaritons
Single-shot Condensation
spellingShingle DRNTU::Science::Physics
Exciton Polaritons
Single-shot Condensation
Snoke, D. W.
Truscott, A. G.
Estrecho, E.
Gao, T.
Bobrovska, N.
Fraser, M. D.
Steger, M.
Pfeiffer, L.
West, K.
Liew, Timothy Chi Hin
Matuszewski, M.
Ostrovskaya, E. A.
Single-shot condensation of exciton polaritons and the hole burning effect
description A bosonic condensate of exciton polaritons in a semiconductor microcavity is a macroscopic quantum state subject to pumping and decay. The fundamental nature of this driven-dissipative condensate is still under debate. Here, we gain an insight into spontaneous condensation by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in a single-shot optical excitation regime, without averaging over multiple condensate realisations. We demonstrate that condensation is strongly influenced by an incoherent reservoir and that the reservoir depletion, the so-called spatial hole burning, is critical for the transition to the ground state. Condensates of photon-like polaritons exhibit strong shot-to-shot fluctuations and density filamentation due to the effective self-focusing associated with the reservoir depletion. In contrast, condensates of exciton-like polaritons display smoother spatial density distributions and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study fundamental properties of non-equilibrium condensation in the presence of a reservoir.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Snoke, D. W.
Truscott, A. G.
Estrecho, E.
Gao, T.
Bobrovska, N.
Fraser, M. D.
Steger, M.
Pfeiffer, L.
West, K.
Liew, Timothy Chi Hin
Matuszewski, M.
Ostrovskaya, E. A.
format Article
author Snoke, D. W.
Truscott, A. G.
Estrecho, E.
Gao, T.
Bobrovska, N.
Fraser, M. D.
Steger, M.
Pfeiffer, L.
West, K.
Liew, Timothy Chi Hin
Matuszewski, M.
Ostrovskaya, E. A.
author_sort Snoke, D. W.
title Single-shot condensation of exciton polaritons and the hole burning effect
title_short Single-shot condensation of exciton polaritons and the hole burning effect
title_full Single-shot condensation of exciton polaritons and the hole burning effect
title_fullStr Single-shot condensation of exciton polaritons and the hole burning effect
title_full_unstemmed Single-shot condensation of exciton polaritons and the hole burning effect
title_sort single-shot condensation of exciton polaritons and the hole burning effect
publishDate 2018
url https://hdl.handle.net/10356/89121
http://hdl.handle.net/10220/46076
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