Spin versus boson baths in nonlinear spectroscopy

The third-order optical response function of a chromophore coupled to a bath consisting of noninteracting two-level systems (TLSs) undergoing stochastic jumps is calculated. The results can be applied to a broad class of nonlinear optical techniques in single-molecule spectroscopy and bulk measureme...

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Bibliographic Details
Main Authors: Zhao, Yang, Chernyak, Vladimir, Mukamel, Shaul
Other Authors: School of Materials Science & Engineering
Format: Article
Language:English
Published: 2011
Subjects:
Online Access:https://hdl.handle.net/10356/93955
http://hdl.handle.net/10220/7419
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Institution: Nanyang Technological University
Language: English
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