Resonant energy transfer assisted by off-diagonal coupling
Dynamics of resonant energy transfer of a single excitation in a molecular dimer system are studied in the simultaneous presence of diagonal and off-diagonal exciton-phonon coupling. It is found that, at given temperatures, the off-diagonal coupling can enhance both the...
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sg-ntu-dr.10356-955832023-07-14T15:53:44Z Resonant energy transfer assisted by off-diagonal coupling Wu, Ning Sun, Kewei Chang, Zhe Zhao, Yang School of Materials Science & Engineering DRNTU::Science::Physics Dynamics of resonant energy transfer of a single excitation in a molecular dimer system are studied in the simultaneous presence of diagonal and off-diagonal exciton-phonon coupling. It is found that, at given temperatures, the off-diagonal coupling can enhance both the coherence of the resonant energy transfer and the net quantity of energy transferred from an initially excited monomer to the other. Also studied is the dynamics of entanglement between the dimer system and the phonon bath as measured by the von Neumann entanglement entropy, and the inter-monomer entanglement dynamics for the excitonic system. Published version 2012-06-25T06:57:51Z 2019-12-06T19:17:52Z 2012-06-25T06:57:51Z 2019-12-06T19:17:52Z 2012 2012 Journal Article Wu, N., Sun, K. W., Chang, Z. & Zhao, Y. (2012). Resonant energy transfer assisted by off-diagonal coupling. The Journal of Chemical Physics, 136(12), 124513-. https://hdl.handle.net/10356/95583 http://hdl.handle.net/10220/8241 10.1063/1.3697817 en The journal of chemical physics © 2012 American Institute of Physics. This paper was published in The Journal of Chemical Physics and is made available as an electronic reprint (preprint) with permission of American Institute of Physics. The paper can be found at the following official URL: [DOI: http://dx.doi.org/10.1063/1.3697817]. One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law. 6 p. application/pdf |
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DRNTU::Science::Physics Wu, Ning Sun, Kewei Chang, Zhe Zhao, Yang Resonant energy transfer assisted by off-diagonal coupling |
description |
Dynamics of resonant energy transfer of a single excitation in a molecular dimer system are studied in
the simultaneous presence of diagonal and off-diagonal exciton-phonon coupling. It is found that, at
given temperatures, the off-diagonal coupling can enhance both the coherence of the resonant energy
transfer and the net quantity of energy transferred from an initially excited monomer to the other. Also
studied is the dynamics of entanglement between the dimer system and the phonon bath as measured
by the von Neumann entanglement entropy, and the inter-monomer entanglement dynamics for the
excitonic system. |
author2 |
School of Materials Science & Engineering |
author_facet |
School of Materials Science & Engineering Wu, Ning Sun, Kewei Chang, Zhe Zhao, Yang |
format |
Article |
author |
Wu, Ning Sun, Kewei Chang, Zhe Zhao, Yang |
author_sort |
Wu, Ning |
title |
Resonant energy transfer assisted by off-diagonal coupling |
title_short |
Resonant energy transfer assisted by off-diagonal coupling |
title_full |
Resonant energy transfer assisted by off-diagonal coupling |
title_fullStr |
Resonant energy transfer assisted by off-diagonal coupling |
title_full_unstemmed |
Resonant energy transfer assisted by off-diagonal coupling |
title_sort |
resonant energy transfer assisted by off-diagonal coupling |
publishDate |
2012 |
url |
https://hdl.handle.net/10356/95583 http://hdl.handle.net/10220/8241 |
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1772827553367588864 |