Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities
CdSxSe1–x nanobelts are interesting nanostructured materials with a tunable band gap from 1.7 to 2.4 eV depending on the nanobelts' stoichiometry. On the basis of their chemical compositions, these nanobelts give out strong photoluminescence with unique color. In this work, we demonstrate that...
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sg-ntu-dr.10356-966362020-06-01T10:01:49Z Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities Lu, Junpeng Lim, Xiaodai Zheng, Minrui Mhaisalkar, Subodh Gautam Sow, Chorng Haur School of Materials Science & Engineering CdSxSe1–x nanobelts are interesting nanostructured materials with a tunable band gap from 1.7 to 2.4 eV depending on the nanobelts' stoichiometry. On the basis of their chemical compositions, these nanobelts give out strong photoluminescence with unique color. In this work, we demonstrate that a direct focused laser beam irradiation was able to achieve localized modification of the chemical composition of the nanobelts. As a result, we could locally change the optical properties of these nanobelts. With a scanning laser beam, micropatterns with a wide range of fluorescence color could be created on a substrate covered with ternary nanobelts without a prepatterned mask. The laser modified nanobelts showed higher resistance to acid corrosion and these nanobelts exhibited more superior photoconductivity. The construction of micropatterns with functionality/color control within the sample would provide greater building blocks for photoelectronic applications. 2013-06-13T03:38:32Z 2019-12-06T19:33:13Z 2013-06-13T03:38:32Z 2019-12-06T19:33:13Z 2012 2012 Journal Article Lu, J., Lim, X., Zheng, M., Mhaisalkar, S. G., & Sow, C.-H. (2012). Direct Laser Pruning of CdSxSe1-x Nanobelts en Route to a Multicolored Pattern with Controlled Functionalities. ACS Nano, 6(9), 8298-8307. 1936-0851 https://hdl.handle.net/10356/96636 http://hdl.handle.net/10220/10312 10.1021/nn303000j en ACS nano © 2012 American Chemical Society. |
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CdSxSe1–x nanobelts are interesting nanostructured materials with a tunable band gap from 1.7 to 2.4 eV depending on the nanobelts' stoichiometry. On the basis of their chemical compositions, these nanobelts give out strong photoluminescence with unique color. In this work, we demonstrate that a direct focused laser beam irradiation was able to achieve localized modification of the chemical composition of the nanobelts. As a result, we could locally change the optical properties of these nanobelts. With a scanning laser beam, micropatterns with a wide range of fluorescence color could be created on a substrate covered with ternary nanobelts without a prepatterned mask. The laser modified nanobelts showed higher resistance to acid corrosion and these nanobelts exhibited more superior photoconductivity. The construction of micropatterns with functionality/color control within the sample would provide greater building blocks for photoelectronic applications. |
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School of Materials Science & Engineering |
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School of Materials Science & Engineering Lu, Junpeng Lim, Xiaodai Zheng, Minrui Mhaisalkar, Subodh Gautam Sow, Chorng Haur |
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Lu, Junpeng Lim, Xiaodai Zheng, Minrui Mhaisalkar, Subodh Gautam Sow, Chorng Haur |
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Lu, Junpeng Lim, Xiaodai Zheng, Minrui Mhaisalkar, Subodh Gautam Sow, Chorng Haur Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
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Lu, Junpeng |
title |
Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
title_short |
Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
title_full |
Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
title_fullStr |
Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
title_full_unstemmed |
Direct laser pruning of CdSxSe1-x nanobelts en route to a multicolored pattern with controlled functionalities |
title_sort |
direct laser pruning of cdsxse1-x nanobelts en route to a multicolored pattern with controlled functionalities |
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2013 |
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https://hdl.handle.net/10356/96636 http://hdl.handle.net/10220/10312 |
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