Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf>
In this paper, we report the dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites consisting of BaTiO3(BT) and 0.975 BaTiO3-0.025Ba (Cu1/3Nb2/3)O3(BTBCN). Two types of graded bilayer samples were synthesized, one with same thickness of BT and BTBCN while ot...
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th-cmuir.6653943832-511592018-09-04T04:52:57Z Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> Deepam Maurya Natthapong Wongdamnern Rattikorn Yimnirun Shashank Priya Physics and Astronomy In this paper, we report the dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites consisting of BaTiO3(BT) and 0.975 BaTiO3-0.025Ba (Cu1/3Nb2/3)O3(BTBCN). Two types of graded bilayer samples were synthesized, one with same thickness of BT and BTBCN while other with different layer thicknesses. The graded trilayer sample consisted of BT layer sandwiched between two BTBCN layers of equal thickness. Scanning electron microscopy and transmission electron microscopy images showed a sharp interface with needle-shape domains across the interface. The domain size on BT side was found to be larger than that on BTBCN side. The temperature dependence of dielectric response for all composite systems was found to exhibit shifting in characteristic Curie peak compared to constituent material which was associated to coupling between layers. Moreover, the differences in grain size, tetragonality, domain mobility of each layer was found to perturb the electrical response of composite. The polarization mismatch between uncoupled BT and BTBCN established internal electric field in composite specimen and defined new polarization states in each layer by perturbing free energy functional of the composite specimen. Dynamic hysteresis behaviors and power-law scaling relations of all specimens were determined from polarization-electric field hysteresis loop measurements as a function of frequency. All systems were found to exhibit similar dynamic scaling relationships. Hysteresis area 〈A〉, Pr, and ECdecreased with increasing frequency due to delayed response but increased with increasing applied electric field due to enhancement of driving force. Trilayer system was found to exhibit strong internal-bias field and double hysteresis behavior. The coupling effect resulting due to polarization mismatch between layers had substantial influence on the dynamic hysteresis behavior and power-law scaling relations. © 2010 American Institute of Physics. 2018-09-04T04:52:57Z 2018-09-04T04:52:57Z 2010-12-15 Journal 00218979 2-s2.0-78650905224 10.1063/1.3514125 https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=78650905224&origin=inward http://cmuir.cmu.ac.th/jspui/handle/6653943832/51159 |
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Physics and Astronomy Deepam Maurya Natthapong Wongdamnern Rattikorn Yimnirun Shashank Priya Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
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In this paper, we report the dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites consisting of BaTiO3(BT) and 0.975 BaTiO3-0.025Ba (Cu1/3Nb2/3)O3(BTBCN). Two types of graded bilayer samples were synthesized, one with same thickness of BT and BTBCN while other with different layer thicknesses. The graded trilayer sample consisted of BT layer sandwiched between two BTBCN layers of equal thickness. Scanning electron microscopy and transmission electron microscopy images showed a sharp interface with needle-shape domains across the interface. The domain size on BT side was found to be larger than that on BTBCN side. The temperature dependence of dielectric response for all composite systems was found to exhibit shifting in characteristic Curie peak compared to constituent material which was associated to coupling between layers. Moreover, the differences in grain size, tetragonality, domain mobility of each layer was found to perturb the electrical response of composite. The polarization mismatch between uncoupled BT and BTBCN established internal electric field in composite specimen and defined new polarization states in each layer by perturbing free energy functional of the composite specimen. Dynamic hysteresis behaviors and power-law scaling relations of all specimens were determined from polarization-electric field hysteresis loop measurements as a function of frequency. All systems were found to exhibit similar dynamic scaling relationships. Hysteresis area 〈A〉, Pr, and ECdecreased with increasing frequency due to delayed response but increased with increasing applied electric field due to enhancement of driving force. Trilayer system was found to exhibit strong internal-bias field and double hysteresis behavior. The coupling effect resulting due to polarization mismatch between layers had substantial influence on the dynamic hysteresis behavior and power-law scaling relations. © 2010 American Institute of Physics. |
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Journal |
author |
Deepam Maurya Natthapong Wongdamnern Rattikorn Yimnirun Shashank Priya |
author_facet |
Deepam Maurya Natthapong Wongdamnern Rattikorn Yimnirun Shashank Priya |
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Deepam Maurya |
title |
Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
title_short |
Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
title_full |
Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
title_fullStr |
Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
title_full_unstemmed |
Dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of BaTiO<inf>3</inf>and 0.975 BaTiO<inf>3</inf>-0.025Ba (Cu<inf>1/3</inf>Nb<inf>2/3</inf>)O<inf>3</inf> |
title_sort |
dielectric and ferroelectric response of compositionally graded bilayer and trilayer composites of batio<inf>3</inf>and 0.975 batio<inf>3</inf>-0.025ba (cu<inf>1/3</inf>nb<inf>2/3</inf>)o<inf>3</inf> |
publishDate |
2018 |
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https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=78650905224&origin=inward http://cmuir.cmu.ac.th/jspui/handle/6653943832/51159 |
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