Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface

Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO3/SrTiO3 heterostructures at previously u...

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Main Authors: David, A., Wu, T., Tsymbal, E. Y., Petrović, A. P., Paré, A., Paudel, T. R., Lee, K., Holmes, S., Barnes, C. H. W., Panagopoulos, C.
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2014
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Online Access:https://hdl.handle.net/10356/104768
http://hdl.handle.net/10220/20281
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Institution: Nanyang Technological University
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spelling sg-ntu-dr.10356-1047682023-02-28T19:42:32Z Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface David, A. Wu, T. Tsymbal, E. Y. Petrović, A. P. Paré, A. Paudel, T. R. Lee, K. Holmes, S. Barnes, C. H. W. Panagopoulos, C. School of Physical and Mathematical Sciences DRNTU::Science::Physics Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO3/SrTiO3 heterostructures at previously unexplored carrier densities n2D ≥ 6.9 × 1014 cm−2, we observe a Shubnikov-de Haas effect for small in-plane fields, characteristic of an anisotropic 3D Fermi surface with preferential dxz,yz orbital occupancy extending over at least 100 nm perpendicular to the interface. Quantum oscillations from the 3D Fermi surface of bulk doped SrTiO3 emerge simultaneously at higher n2D. We distinguish three areas in doped perovskite heterostructures: narrow (<20 nm) 2D interfaces housing superconductivity and/or other emergent phases, electronically isotropic regions far (>120 nm) from the interface and new intermediate zones where interfacial proximity renormalises the electronic structure relative to the bulk. Published version 2014-08-14T08:43:24Z 2019-12-06T21:39:17Z 2014-08-14T08:43:24Z 2019-12-06T21:39:17Z 2014 2014 Journal Article Petrović, A. P., Paré, A., Paudel, T. R., Lee, K., Holmes, S., Barnes, C. H. W., et al. (2014). Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface. Scientific Reports, 4-. 2045-2322 https://hdl.handle.net/10356/104768 http://hdl.handle.net/10220/20281 10.1038/srep05338 24939804 en Scientific reports This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder in order to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/4.0/ application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic DRNTU::Science::Physics
spellingShingle DRNTU::Science::Physics
David, A.
Wu, T.
Tsymbal, E. Y.
Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
Panagopoulos, C.
Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
description Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO3/SrTiO3 heterostructures at previously unexplored carrier densities n2D ≥ 6.9 × 1014 cm−2, we observe a Shubnikov-de Haas effect for small in-plane fields, characteristic of an anisotropic 3D Fermi surface with preferential dxz,yz orbital occupancy extending over at least 100 nm perpendicular to the interface. Quantum oscillations from the 3D Fermi surface of bulk doped SrTiO3 emerge simultaneously at higher n2D. We distinguish three areas in doped perovskite heterostructures: narrow (<20 nm) 2D interfaces housing superconductivity and/or other emergent phases, electronically isotropic regions far (>120 nm) from the interface and new intermediate zones where interfacial proximity renormalises the electronic structure relative to the bulk.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
David, A.
Wu, T.
Tsymbal, E. Y.
Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
Panagopoulos, C.
format Article
author David, A.
Wu, T.
Tsymbal, E. Y.
Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
Panagopoulos, C.
author_sort David, A.
title Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
title_short Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
title_full Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
title_fullStr Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
title_full_unstemmed Long-range electronic reconstruction to a dxz,yz-dominated Fermi surface below the LaAlO3/SrTiO3 interface
title_sort long-range electronic reconstruction to a dxz,yz-dominated fermi surface below the laalo3/srtio3 interface
publishDate 2014
url https://hdl.handle.net/10356/104768
http://hdl.handle.net/10220/20281
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