Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface

The quasi-two-dimensional electron gas at oxide interfaces provides a platform for investigating quantum phenomena in strongly correlated electronic systems. Here, we study the transport properties at the high-mobility (La0.3Sr0.7) (Al0.65Ta0.35) O3/SrTiO3 interface. Before oxygen annealing, the as-...

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التفاصيل البيبلوغرافية
المؤلفون الرئيسيون: Han, K., Huang, Z., Zeng, S. W., Yang, M., Li, C. J., Zhou, W. X., Wang, Renshaw Xiao, Venkatesan, T., Coey, J. M. D., Goiran, M., Escoffier, W., Ariando
مؤلفون آخرون: School of Electrical and Electronic Engineering
التنسيق: مقال
اللغة:English
منشور في: 2019
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الوصول للمادة أونلاين:https://hdl.handle.net/10356/106772
http://hdl.handle.net/10220/48973
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spelling sg-ntu-dr.10356-1067722023-02-28T19:45:53Z Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface Han, K. Huang, Z. Zeng, S. W. Yang, M. Li, C. J. Zhou, W. X. Wang, Renshaw Xiao Venkatesan, T. Coey, J. M. D. Goiran, M. Escoffier, W. Ariando School of Electrical and Electronic Engineering School of Physical and Mathematical Sciences Electronic Structure Hall Effect DRNTU::Science::Physics The quasi-two-dimensional electron gas at oxide interfaces provides a platform for investigating quantum phenomena in strongly correlated electronic systems. Here, we study the transport properties at the high-mobility (La0.3Sr0.7) (Al0.65Ta0.35) O3/SrTiO3 interface. Before oxygen annealing, the as-grown interface exhibits a high electron density and electron occupancy of two subbands: higher-mobility electrons (μ1≈10^4 cm2 V−1s−1 at 2 K) occupy the lower-energy 3dxy subband, while lower-mobility electrons (μ1≈103cm2V−1s−1 at 2 K) propagate in the higher-energy 3dxz/yz-dominated subband. After removing oxygen vacancies by annealing in oxygen, only a single type of 3dxy electrons remain at the annealed interface, showing tunable Shubnikov–de Haas oscillations below 9 T at 2 K and an effective mass of 0.7me. By contrast, no oscillation is observed at the as-grown interface even when electron mobility is increased to 50 000 cm2V−1s−1 by gating voltage. Our results reveal the important roles of both carrier mobility and subband occupancy in tuning the quantum transport at oxide interfaces. NRF (Natl Research Foundation, S’pore) MOE (Min. of Education, S’pore) Published version 2019-06-27T02:35:56Z 2019-12-06T22:18:08Z 2019-06-27T02:35:56Z 2019-12-06T22:18:08Z 2017 Journal Article Han, K., Huang, Z., Zeng, S. W., Yang, M., Li, C. J., Zhou, W. X., . . . Ariando. (2017). Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface. Physical Review Materials, 1(1), 011601-. doi:10.1103/PhysRevMaterials.1.011601 https://hdl.handle.net/10356/106772 http://hdl.handle.net/10220/48973 10.1103/PhysRevMaterials.1.011601 en Physical Review Materials © 2017 American Physical Society. All rights reserved. This paper was published in Physical Review Materials and is made available with permission of American Physical Society. 6 p. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Electronic Structure
Hall Effect
DRNTU::Science::Physics
spellingShingle Electronic Structure
Hall Effect
DRNTU::Science::Physics
Han, K.
Huang, Z.
Zeng, S. W.
Yang, M.
Li, C. J.
Zhou, W. X.
Wang, Renshaw Xiao
Venkatesan, T.
Coey, J. M. D.
Goiran, M.
Escoffier, W.
Ariando
Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
description The quasi-two-dimensional electron gas at oxide interfaces provides a platform for investigating quantum phenomena in strongly correlated electronic systems. Here, we study the transport properties at the high-mobility (La0.3Sr0.7) (Al0.65Ta0.35) O3/SrTiO3 interface. Before oxygen annealing, the as-grown interface exhibits a high electron density and electron occupancy of two subbands: higher-mobility electrons (μ1≈10^4 cm2 V−1s−1 at 2 K) occupy the lower-energy 3dxy subband, while lower-mobility electrons (μ1≈103cm2V−1s−1 at 2 K) propagate in the higher-energy 3dxz/yz-dominated subband. After removing oxygen vacancies by annealing in oxygen, only a single type of 3dxy electrons remain at the annealed interface, showing tunable Shubnikov–de Haas oscillations below 9 T at 2 K and an effective mass of 0.7me. By contrast, no oscillation is observed at the as-grown interface even when electron mobility is increased to 50 000 cm2V−1s−1 by gating voltage. Our results reveal the important roles of both carrier mobility and subband occupancy in tuning the quantum transport at oxide interfaces.
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Han, K.
Huang, Z.
Zeng, S. W.
Yang, M.
Li, C. J.
Zhou, W. X.
Wang, Renshaw Xiao
Venkatesan, T.
Coey, J. M. D.
Goiran, M.
Escoffier, W.
Ariando
format Article
author Han, K.
Huang, Z.
Zeng, S. W.
Yang, M.
Li, C. J.
Zhou, W. X.
Wang, Renshaw Xiao
Venkatesan, T.
Coey, J. M. D.
Goiran, M.
Escoffier, W.
Ariando
author_sort Han, K.
title Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
title_short Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
title_full Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
title_fullStr Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
title_full_unstemmed Electrical properties and subband occupancy at the (La, Sr)(Al, Ta)O3/SrTiO3 interface
title_sort electrical properties and subband occupancy at the (la, sr)(al, ta)o3/srtio3 interface
publishDate 2019
url https://hdl.handle.net/10356/106772
http://hdl.handle.net/10220/48973
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