Giant hall photoconductivity in narrow-gapped dirac materials

Carrier dynamics acquire a new character in the presence of Bloch-band Berry curvature, which naturally arises in gapped Dirac materials (GDMs). Here, we argue that photoresponse in GDMs with small band gaps is dramatically enhanced by Berry curvature. This manifests in a giant and saturable Hall ph...

Full description

Saved in:
Bibliographic Details
Main Authors: Song, Justin Chien Wen, Kats, Mikhail A.
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/137991
Tags: Add Tag
No Tags, Be the first to tag this record!
Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-137991
record_format dspace
spelling sg-ntu-dr.10356-1379912023-02-28T19:49:43Z Giant hall photoconductivity in narrow-gapped dirac materials Song, Justin Chien Wen Kats, Mikhail A. School of Physical and Mathematical Sciences Institute of High Performance Computing, A*STAR Science::Physics Photoconductivity Two-dimensional Materials Carrier dynamics acquire a new character in the presence of Bloch-band Berry curvature, which naturally arises in gapped Dirac materials (GDMs). Here, we argue that photoresponse in GDMs with small band gaps is dramatically enhanced by Berry curvature. This manifests in a giant and saturable Hall photoconductivity when illuminated by circularly polarized light. Unlike Hall motion arising from a Lorentz force in a magnetic field, which impedes longitudinal carrier motion, Hall photoconductivity arising from Berry curvature can boost longitudinal carrier transport. In GDMs, this results in a helicity-dependent photoresponse in the Hall regime, where photoconductivity is dominated by its Hall component. We find that the induced Hall conductivity per incident irradiance is enhanced by up to 6 orders of magnitude when moving from the visible regime (with corresponding band gaps) to the far infrared. These results suggest that narrow-gap GDMs are an ideal test-bed for the unique physics that arise in the presence of Berry curvature and open a new avenue for infrared and terahertz optoelectronics. NRF (Natl Research Foundation, S’pore) Accepted version 2020-04-21T07:34:46Z 2020-04-21T07:34:46Z 2016 Journal Article Song, J. C. W., & Kats, M. A. (2016). Giant hall photoconductivity in narrow-gapped dirac materials. Nano Letters, 16(12), 7346−7351. doi:10.1021/acs.nanolett.6b02559 1530-6984 https://hdl.handle.net/10356/137991 10.1021/acs.nanolett.6b02559 27960456 2-s2.0-85006306454 12 16 7346 7351 en Nano Letters This document is the Accepted Manuscript version of a Published Work that appeared in final form in Nano Letters, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.nanolett.6b02559 application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics
Photoconductivity
Two-dimensional Materials
spellingShingle Science::Physics
Photoconductivity
Two-dimensional Materials
Song, Justin Chien Wen
Kats, Mikhail A.
Giant hall photoconductivity in narrow-gapped dirac materials
description Carrier dynamics acquire a new character in the presence of Bloch-band Berry curvature, which naturally arises in gapped Dirac materials (GDMs). Here, we argue that photoresponse in GDMs with small band gaps is dramatically enhanced by Berry curvature. This manifests in a giant and saturable Hall photoconductivity when illuminated by circularly polarized light. Unlike Hall motion arising from a Lorentz force in a magnetic field, which impedes longitudinal carrier motion, Hall photoconductivity arising from Berry curvature can boost longitudinal carrier transport. In GDMs, this results in a helicity-dependent photoresponse in the Hall regime, where photoconductivity is dominated by its Hall component. We find that the induced Hall conductivity per incident irradiance is enhanced by up to 6 orders of magnitude when moving from the visible regime (with corresponding band gaps) to the far infrared. These results suggest that narrow-gap GDMs are an ideal test-bed for the unique physics that arise in the presence of Berry curvature and open a new avenue for infrared and terahertz optoelectronics.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Song, Justin Chien Wen
Kats, Mikhail A.
format Article
author Song, Justin Chien Wen
Kats, Mikhail A.
author_sort Song, Justin Chien Wen
title Giant hall photoconductivity in narrow-gapped dirac materials
title_short Giant hall photoconductivity in narrow-gapped dirac materials
title_full Giant hall photoconductivity in narrow-gapped dirac materials
title_fullStr Giant hall photoconductivity in narrow-gapped dirac materials
title_full_unstemmed Giant hall photoconductivity in narrow-gapped dirac materials
title_sort giant hall photoconductivity in narrow-gapped dirac materials
publishDate 2020
url https://hdl.handle.net/10356/137991
_version_ 1759855938945155072