Dynamic assembly of active matter

Active matter refers to particles that can dissipate energy and drive their own motion. They display intriguing dynamic assembly phenomena as not restricted by equilibrium thermodynamics, including motility-induced phase separation (MIPS), collective motion, giant number fluctuation, and formation o...

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Main Author: Ma, Zhan
Other Authors: Ni Ran
Format: Thesis-Doctor of Philosophy
Language:English
Published: Nanyang Technological University 2021
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Online Access:https://hdl.handle.net/10356/151042
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Institution: Nanyang Technological University
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spelling sg-ntu-dr.10356-1510422021-07-08T16:01:18Z Dynamic assembly of active matter Ma, Zhan Ni Ran School of Chemical and Biomedical Engineering r.ni@ntu.edu.sg Engineering::Bioengineering Active matter refers to particles that can dissipate energy and drive their own motion. They display intriguing dynamic assembly phenomena as not restricted by equilibrium thermodynamics, including motility-induced phase separation (MIPS), collective motion, giant number fluctuation, and formation of complex patterns, etc. The study of dynamic assembly of active matter can help both understand the emergent behavior in living creatures and design dynamic materials. Multiple models have been proposed to study active matters, such as active Brownian particles (ABPs) and Vicsek-like models. However, most of these models ignore the intrinsic trajectory curvature and chiral swimming pattern, which are widely observed in active matter systems. This thesis focuses on the phase behavior of circle swimmers. We construct the circle active Brownian particles (cABPs) model by introducing the self-propulsion torque. Then we formulate a continuum theory for cABPs, and the fluctuation dispersion relation reveals two types of instabilities of the homogeneous state. Compared with simulations results, we verify that the type I instability leads to MIPS, while the type II instability, also called finite wave-number instability, results in a dynamic clustering state and interrupts the conventional MIPS. Besides, by measuring the self-intermediate scattering function, we reveal the dynamical property of this novel inhomogeneous state. Along with obtaining the full phase diagram of cABPs, we also study the phase transition between homogeneous state and dynamic clustering state in the context of percolation theory. Finally, we find the spontaneous demixing of circle swimmers and passive particles, which may have potential application in collecting and sorting passive colloids. Doctor of Philosophy 2021-06-23T05:04:08Z 2021-06-23T05:04:08Z 2021 Thesis-Doctor of Philosophy Ma, Z. (2021). Dynamic assembly of active matter. Doctoral thesis, Nanyang Technological University, Singapore. https://hdl.handle.net/10356/151042 https://hdl.handle.net/10356/151042 10.32657/10356/151042 en MOE2019-T2-2-010 M4081781.120 RG104/17(S) A1784C0018 M4011616.120 M4011873.120 10.1039/c7sm01730h 10.1002/adts.202000021 This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License (CC BY-NC 4.0). application/pdf Nanyang Technological University
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Bioengineering
spellingShingle Engineering::Bioengineering
Ma, Zhan
Dynamic assembly of active matter
description Active matter refers to particles that can dissipate energy and drive their own motion. They display intriguing dynamic assembly phenomena as not restricted by equilibrium thermodynamics, including motility-induced phase separation (MIPS), collective motion, giant number fluctuation, and formation of complex patterns, etc. The study of dynamic assembly of active matter can help both understand the emergent behavior in living creatures and design dynamic materials. Multiple models have been proposed to study active matters, such as active Brownian particles (ABPs) and Vicsek-like models. However, most of these models ignore the intrinsic trajectory curvature and chiral swimming pattern, which are widely observed in active matter systems. This thesis focuses on the phase behavior of circle swimmers. We construct the circle active Brownian particles (cABPs) model by introducing the self-propulsion torque. Then we formulate a continuum theory for cABPs, and the fluctuation dispersion relation reveals two types of instabilities of the homogeneous state. Compared with simulations results, we verify that the type I instability leads to MIPS, while the type II instability, also called finite wave-number instability, results in a dynamic clustering state and interrupts the conventional MIPS. Besides, by measuring the self-intermediate scattering function, we reveal the dynamical property of this novel inhomogeneous state. Along with obtaining the full phase diagram of cABPs, we also study the phase transition between homogeneous state and dynamic clustering state in the context of percolation theory. Finally, we find the spontaneous demixing of circle swimmers and passive particles, which may have potential application in collecting and sorting passive colloids.
author2 Ni Ran
author_facet Ni Ran
Ma, Zhan
format Thesis-Doctor of Philosophy
author Ma, Zhan
author_sort Ma, Zhan
title Dynamic assembly of active matter
title_short Dynamic assembly of active matter
title_full Dynamic assembly of active matter
title_fullStr Dynamic assembly of active matter
title_full_unstemmed Dynamic assembly of active matter
title_sort dynamic assembly of active matter
publisher Nanyang Technological University
publishDate 2021
url https://hdl.handle.net/10356/151042
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