Single-Ni sites embedded in multilayer nitrogen-doped graphene derived from amino-functionalized MOF for highly selective CO₂ electroreduction

• Main Authors: Wang, Haojing, Liu, Guanyu, Chen, Chunping, Tu, Wenguang, Lu, Yan, Wu, Shuyang, O'Hare, Dermot, Xu, Rong
• Other Authors: School of Chemical and Biomedical Engineering
• Format: Article
• Language: English
• Published: 2022
• Subjects: Engineering::Chemical engineering; Electrocatalysis; Metal−Organic Framework
• Online Access: https://hdl.handle.net/10356/159950
• Institution: Nanyang Technological University

CO2 electroreduction using renewable electricity is a promising pathway for CO2 utilization. However, the development of highly active and selective catalysts for CO2 reduction still poses significant challenges. Here, we report the use of an amino-functionalized metal-organic framework as a precurs...